Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Optical Injection and Detection of Long-Lived Interlayer Excitons in van der Waals Heterostructures

Alperen Tüğen1,*, Anna M. Seiler1,*, Arthur Christianen1, Kenji Watanabe2, Takashi Taniguchi3, Martin Kroner1, and Ataç İmamoğlu1

  • *These authors contributed equally to this work.

Phys. Rev. Lett. 135, 246502 – Published 10 December, 2025

DOI: https://doi.org/10.1103/stgs-2s58

Abstract

Interlayer excitons in semiconducting bilayers separated by insulating hexagonal boron nitride (h-BN) layers constitute a promising platform for investigation of strongly correlated bosonic phases. Here, we report an optical method for the generation and characterization of long-lived interlayer excitons. We confirm the presence of tightly bound interlayer excitons by measuring 1s and 2s intralayer excitons in each layer concurrently. Using a pump-probe technique, we find interlayer exciton lifetimes up to 8.8  μs, increasing with the thickness of the h-BN. With optical access to long-lived interlayer excitons, our approach provides a new route to explore degenerate Bose–Fermi mixtures of excitons and itinerant electrons with high spatial and temporal resolution.

View figure in article

Physics Subject Headings (PhySH)

Article Text

Supplemental Material

References (45)

  1. M. Lu, N. Q. Burdick, S. H. Youn, and B. L. Lev, Phys. Rev. Lett. 107, 190401 (2011).
  2. K. Aikawa, A. Frisch, M. Mark, S. Baier, A. Rietzler, R. Grimm, and F. Ferlaino, Phys. Rev. Lett. 108, 210401 (2012).
  3. M. Alloing, M. Beian, M. Lewenstein, D. Fuster, Y. González, L. González, R. Combescot, M. Combescot, and F. Dubin, Europhys. Lett. 107, 10012 (2014).
  4. M. Combescot, R. Combescot, and F. Dubin, Rep. Prog. Phys. 80, 066501 (2017).
  5. C. Zerba, C. Kuhlenkamp, A. Imamoǧlu, and M. Knap, Phys. Rev. Lett. 133, 056902 (2024).
  6. J. von Milczewski, X. Chen, A. Imamoglu, and R. Schmidt, Phys. Rev. Lett. 133, 226903 (2024).
  7. A. A. High, J. R. Leonard, A. T. Hammack, M. M. Fogler, L. V. Butov, A. V. Kavokin, K. L. Campman, and A. C. Gossard, Nature (London) 483, 584 (2012).
  8. L. Ma, P. X. Nguyen, Z. Wang, Y. Zeng, K. Watanabe, T. Taniguchi, A. H. MacDonald, K. F. Mak, and J. Shan, Nature (London) 598, 585 (2021).
  9. R. Qi, A. Y. Joe, Z. Zhang, Y. Zeng, T. Zheng, Q. Feng, J. Xie, E. Regan, Z. Lu, T. Taniguchi, K. Watanabe, S. Tongay, M. F. Crommie, A. H. MacDonald, and F. Wang, Nat. Commun. 14, 8264 (2023).
  10. P. X. Nguyen, L. Ma, R. Chaturvedi, K. Watanabe, T. Taniguchi, J. Shan, and K. F. Mak, Science 388, 274 (2025).
  11. R. Qi, A. Y. Joe, Z. Zhang, J. Xie, Q. Feng, Z. Lu, Z. Wang, T. Taniguchi, K. Watanabe, S. Tongay, and F. Wang, Science 388, 278 (2025).
  12. P. Rivera, J. R. Schaibley, A. M. Jones, J. S. Ross, S. Wu, G. Aivazian, P. Klement, K. Seyler, G. Clark, N. J. Ghimire et al., Nat. Commun. 6, 6242 (2015).
  13. L. A. Jauregui, A. Y. Joe, K. Pistunova, D. S. Wild, A. A. High, Y. Zhou, G. Scuri, K. De Greve, A. Sushko, C.-H. Yu et al., Science 366, 870 (2019).
  14. Y. Shimazaki, I. Schwartz, K. Watanabe, T. Taniguchi, M. Kroner, and A. Imamoǧlu, Nature (London) 580, 472 (2020).
  15. F. Mahdikhanysarvejahany, D. N. Shanks, M. Klein, Q. Wang, M. R. Koehler, D. G. Mandrus, T. Taniguchi, K. Watanabe, O. L. Monti, B. J. LeRoy et al., Nat. Commun. 13, 5354 (2022).
  16. J. Cutshall, F. Mahdikhany, A. Roche, D. N. Shanks, M. R. Koehler, D. G. Mandrus, T. Taniguchi, K. Watanabe, Q. Zhu, B. J. LeRoy et al., Sci. Adv. 11, eadr1772 (2025).
  17. D. Snoke, Adv. Condens. Matter Phys. 2011, 938609 (2011).
  18. See Supplemental Material at http://link.aps.org/supplemental/10.1103/stgs-2s58 for experimental details, additional figures and further discussion, which includes Refs. [19–27].
  19. A. Reinhard, Strong photon-photon interactions in solid state cavity QED, Ph.D. thesis, ETH Zurich, 2013.
  20. J. G. Roch, D. Miserev, G. Froehlicher, N. Leisgang, L. Sponfeldner, K. Watanabe, T. Taniguchi, J. Klinovaja, D. Loss, and R. J. Warburton, Phys. Rev. Lett. 124, 187602 (2020).
  21. T. Wang, Z. Li, Z. Lu, Y. Li, S. Miao, Z. Lian, Y. Meng, M. Blei, T. Taniguchi, K. Watanabe et al., Phys. Rev. X 10, 021024 (2020).
  22. E. Liu, J. van Baren, T. Taniguchi, K. Watanabe, Y.-C. Chang, and C. H. Lui, Phys. Rev. B 99, 205420 (2019).
  23. T. Smoleński, O. Cotlet, A. Popert, P. Back, Y. Shimazaki, P. Knüppel, N. Dietler, T. Taniguchi, K. Watanabe, M. Kroner et al., Phys. Rev. Lett. 123, 097403 (2019).
  24. J. Kang, S. Tongay, J. Zhou, J. Li, and J. Wu, Appl. Phys. Lett. 102, 012111 (2013).
  25. P. Rivera, H. Yu, K. L. Seyler, N. P. Wilson, W. Yao, and X. Xu, Nat. Nanotechnol. 13, 1004 (2018).
  26. Y. Yoon, Z. Zhang, R. Qi, A. Y. Joe, R. Sailus, K. Watanabe, T. Taniguchi, S. Tongay, and F. Wang, Nano Lett. 22, 10140 (2022).
  27. T. Handa, M. Holbrook, N. Olsen, L. N. Holtzman, L. Huber, H. I. Wang, M. Bonn, K. Barmak, J. C. Hone, A. N. Pasupathy et al., Sci. Adv. 10, eadj4060 (2024).
  28. Device 1 shows very weak interlayer PL, whereas no interlayer PL is observed in Device 2 or 3; see Fig. S2 in Supplemental Material [18].

  29. M. Sidler, P. Back, O. Cotlet, A. Srivastava, T. Fink, M. Kroner, E. Demler, and A. Imamoglu, Nat. Phys. 13, 255 (2017).
  30. We emphasize that the two types of doping can be spectrally distinguished in WSe2 [21]: the presence of a single attractive polaron (AP) resonance in the WSe2 spectrum unequivocally indicates hole doping since electron doping of WSe2 leads to two AP features associated with the singlet and triplet trions. By contrast, MoSe2 displays a single AP peak under both electron and hole doping. Additional confirmation comes from Device 3, a MoS2/WSe2 heterostructure, where the MoS2 layer clearly exhibits two AP features under electron doping, consistent with our interpretation of the spectra in Devices 1 and 2 (see Fig. S6 [18]).

  31. I. Amelio, N. D. Drummond, E. Demler, R. Schmidt, and A. Imamoglu, Phys. Rev. B 107, 155303.
  32. Y. Xu, S. Liu, D. A. Rhodes, K. Watanabe, T. Taniguchi, J. Hone, V. Elser, K. F. Mak, and J. Shan, Nature (London) 587, 214 (2020).
  33. A. Popert, Y. Shimazaki, M. Kroner, K. Watanabe, T. Taniguchi, A. Imamoǧlu, and T. Smoleński, Nano Lett. 22, 7363 (2022).
  34. J. Kim, H. Dery, and D. Van Tuan, Phys. Rev. B 112, L041301 (2025).
  35. A. Christianen, A. M. Seiler, A. Tüǧen, and A. İmamoǧlu (to be published).
  36. N. Kiper, H. S. Adlong, A. Christianen, M. Kroner, K. Watanabe, T. Taniguchi, and A. İmamoǧlu, Phys. Rev. X 15, 011049 (2025).
  37. The parabolic trend in the logarithmic plot in Fig. 4 is clearly visible; similar nonexponential time dependence has also been observed by Cutshall et al. [16] in a time-resolved PL measurement.

  38. T. Uto, B. Evrard, K. Watanabe, T. Taniguchi, M. Kroner, and A. İmamoǧlu, Phys. Rev. Lett. 132, 056901 (2024).
  39. B. Khorana, Phys. Rev. 185, 299 (1969).
  40. K. G. Lagoudakis, B. Pietka, M. Wouters, R. André, and B. Deveaud-Plédran, Phys. Rev. Lett. 105, 120403 (2010).
  41. M. Abbarchi, A. Amo, V. Sala, D. Solnyshkov, H. Flayac, L. Ferrier, I. Sagnes, E. Galopin, A. Lemaître, G. Malpuech et al., Nat. Phys. 9, 275 (2013).
  42. R. Rapaport, G. Chen, S. Simon, O. Mitrofanov, L. Pfeiffer, and P. M. Platzman, Phys. Rev. B 72, 075428 (2005).
  43. A. Gärtner, L. Prechtel, D. Schuh, A. W. Holleitner, and J. P. Kotthaus, Phys. Rev. B 76, 085304 (2007).
  44. E. C. Regan, D. Wang, C. Jin, M. I. Bakti Utama, B. Gao, X. Wei, S. Zhao, W. Zhao, Z. Zhang, K. Yumigeta et al., Nature (London) 579, 359 (2020).
  45. A. Tüǧen and A. M. Seiler, 2025, 10.3929/ethz-c-000785878.

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation