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    Ferromagnetic Interface Engineering of Spin-Charge Conversion in RuO2

    Dongchao Yang1, Zhaoqing Li2, Yu Dai3, Lili Lang4, Zhong Shi1,*, Zhe Yuan2,†, and Shi-Ming Zhou1

    • *Contact author: shizhong@tongji.edu.cn
    • †Contact author: yuanz@fudan.edu.cn

    Phys. Rev. Lett. 136, 026702 – Published 14 January, 2026

    DOI: https://doi.org/10.1103/rc4k-rf1p

    Abstract

    Spin-orbit torque efficiency is conventionally fixed by bulk materials. D-wave altermagnets introduce an additional nonrelativistic spin-charge conversion channel beyond the inverse spin-Hall effect. Using prototypical candidate RuO2 as an example, we show that the adjacent ferromagnet alone can dictate both the magnitude and sign of spin-charge conversion. Spin-pumping measurements on RuO2/Y3Fe5O12 (YIG) and RuO2/Ni80Fe20 (Py) bilayers yield opposite effective spin-Hall angles that persist across crystalline and polycrystalline RuO2. Inserting an ultrathin Au spacer at the RuO2/YIG interface reverses the signal, evidencing a dominant interfacial inverse Rashba-Edelstein effect, whereas RuO2/Py is governed by the bulk inverse spin-Hall effect. First-principles calculations trace this dichotomy to interface-selective band hybridization: Rashba surface states survive at the insulating YIG contact yet are quenched by metallic Py. Our findings establish ferromagnetic interfacing as a deterministic knob for tailoring spin-charge conversion in altermagnetic oxides, paving the way to field-free, low-dissipation spintronic memory devices.

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