Ferromagnetic Interface Engineering of Spin-Charge Conversion in
Phys. Rev. Lett. 136, 026702 – Published 14 January, 2026
DOI: https://doi.org/10.1103/rc4k-rf1p
Abstract
Spin-orbit torque efficiency is conventionally fixed by bulk materials. -wave altermagnets introduce an additional nonrelativistic spin-charge conversion channel beyond the inverse spin-Hall effect. Using prototypical candidate as an example, we show that the adjacent ferromagnet alone can dictate both the magnitude and sign of spin-charge conversion. Spin-pumping measurements on (YIG) and (Py) bilayers yield opposite effective spin-Hall angles that persist across crystalline and polycrystalline . Inserting an ultrathin Au spacer at the interface reverses the signal, evidencing a dominant interfacial inverse Rashba-Edelstein effect, whereas is governed by the bulk inverse spin-Hall effect. First-principles calculations trace this dichotomy to interface-selective band hybridization: Rashba surface states survive at the insulating YIG contact yet are quenched by metallic Py. Our findings establish ferromagnetic interfacing as a deterministic knob for tailoring spin-charge conversion in altermagnetic oxides, paving the way to field-free, low-dissipation spintronic memory devices.