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    Electronic Layer Decoupling Driven by Density-Wave Order in La4Ni3O10

    Ziqiang Guan (管梓强)1,*, Sophia F. R. TenHuisen1,2,*, M. Tepie1, Yifeng Zhao (赵祎峰)3, Ezra Day-Roberts3, Harrison LaBollita3, Alexander M. Young1, Xiaomeng Cui (崔宵萌)1, Xinglong Chen (陈幸龙)4 et al.

    Filippo Glerean1,5, Carl Audric Guia1, Mark P. M. Dean5, Philip Kim1,2, J. F. Mitchell4, Antia S. Botana3, Christopher C. Homes6, and Matteo Mitrano1,†

    • *These authors contributed equally to this work.
    • †Contact author: mmitrano@g.harvard.edu

    Phys. Rev. Lett. 136, 216501 – Published 26 May, 2026

    DOI: https://doi.org/10.1103/qgl1-zh9f

    Abstract

    We probe the density-wave transition of the trilayer nickelate La4Ni3O10 with polarization-resolved infrared spectroscopy. The low-energy electrodynamics is strongly anisotropic, with metallic in-plane and insulating out-of-plane character. In the ordered phase, the anisotropy grows more than an order of magnitude as the out-of-plane conductivity is sharply suppressed. We interpret this enhancement as an effective electronic decoupling of the Ni-O layers driven by a spin-density-wave-induced redistribution of Ni−dz2 occupation within the trilayers. This electronic response is accompanied by clearly shifting and splitting out-of-plane phonons, compatible with a density-wave instability of electronic origin.

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