Electronic Layer Decoupling Driven by Density-Wave Order in
Phys. Rev. Lett. 136, 216501 – Published 26 May, 2026
DOI: https://doi.org/10.1103/qgl1-zh9f
Abstract
We probe the density-wave transition of the trilayer nickelate with polarization-resolved infrared spectroscopy. The low-energy electrodynamics is strongly anisotropic, with metallic in-plane and insulating out-of-plane character. In the ordered phase, the anisotropy grows more than an order of magnitude as the out-of-plane conductivity is sharply suppressed. We interpret this enhancement as an effective electronic decoupling of the Ni-O layers driven by a spin-density-wave-induced redistribution of occupation within the trilayers. This electronic response is accompanied by clearly shifting and splitting out-of-plane phonons, compatible with a density-wave instability of electronic origin.