Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Strain-Controlled Atomic Reconstruction and Quasi-1D Excitons in Moiré Heterostructures

Shen Zhao1,2,*, Zhijie Li1, Zakhar A. Iakovlev3, Peirui Ji4, Tao Jiang5, Fanrong Lin6, Xin Huang7, Kenji Watanabe8, Takashi Taniguchi9 et al.

Mikhail M. Glazov3, Anvar S. Baimuratov1,10,†, and Alexander Högele1,11,‡

  • *Contact author: szhao@nju.edu.cn
  • Contact author: a.baimuratov@skoltech.ru
  • Contact author: alexander.hoegele@lmu.de

Phys. Rev. Lett. 136, 176201 – Published 30 April, 2026

DOI: https://doi.org/10.1103/qdq1-2yk9

Abstract

In two-dimensional materials, strain provides effective means for tailoring electronic and optical properties. While uni- or biaxial strain has been widely implemented in monolayer semiconductors, deterministic control over atomic reconstruction and the resulting microscopic stacking textures in moiré heterostructures remains challenging. Here, we demonstrate the controlled formation of one-dimensional quantum wire arrays in MoSe2WSe2 heterobilayers through the interplay of uniaxial strain and atomic reconstruction. This process yields one-dimensional confinement of interlayer excitons within domain walls, producing near-unity linearly polarized emission due to confinement-induced symmetry breaking. The domain wall width and thereby the degree of exciton confinement can be precisely tuned via the interlayer twist angle. Under an out-of-plane electric field, the confined excitons exhibit Stark shifts exceeding 100 meV and fine-structure splitting modulations by up to a factor of 2. These findings establish strain tuning as a powerful route to realize designer moiré systems with programmable quantum properties, opening new opportunities for optoelectronic applications.

View figure in article

Physics Subject Headings (PhySH)

Article Text

Supplemental Material

References (55)

  1. K. P. Nuckolls and A. Yazdani, A microscopic perspective on moiré materials, Nat. Rev. Mater. 9, 460 (2024).
  2. F. Escudero, A. Sinner, Z. Zhan, P. A. Pantaleón, and F. Guinea, Designing moiré patterns by strain, Phys. Rev. Res. 6, 023203 (2024).
  3. M. Kögl, P. Soubelet, M. Brotons-Gisbert, A. V. Stier, B. D. Gerardot, and J. J. Finley, Moiré straintronics: A universal platform for reconfigurable quantum materials, npj 2D Mater. Appl. 7, 32 (2023).
  4. H. Yoo, R. Engelke, S. Carr, S. Fang, K. Zhang, P. Cazeaux, S. H. Sung, R. Hovden, A. W. Tsen, T. Taniguchi, K. Watanabe, G.-C. Yi, M. Kim, M. Luskin, E. B. Tadmor, E. Kaxiras, and P. Kim, Atomic and electronic reconstruction at the van der Waals interface in twisted bilayer graphene, Nat. Mater. 18, 448 (2019).
  5. A. Weston et al., Atomic reconstruction in twisted bilayers of transition metal dichalcogenides, Nat. Nanotechnol. 15, 592 (2020).
  6. N. P. Kazmierczak, M. Van Winkle, C. Ophus, K. C. Bustillo, S. Carr, H. G. Brown, J. Ciston, T. Taniguchi, K. Watanabe, and D. K. Bediako, Strain fields in twisted bilayer graphene, Nat. Mater. 20, 956 (2021).
  7. D. Halbertal et al., Moiré metrology of energy landscapes in van der Waals heterostructures, Nat. Commun. 12, 242 (2021).
  8. T. A. de Jong, T. Benschop, X. Chen, E. E. Krasovskii, M. J. A. de Dood, R. M. Tromp, M. P. Allan, and S. J. van der Molen, Imaging moiré deformation and dynamics in twisted bilayer graphene, Nat. Commun. 13, 70 (2022).
  9. D. Halbertal, S. Turkel, C. J. Ciccarino, J. B. Profe, N. Finney, V. Hsieh, K. Watanabe, T. Taniguchi, J. Hone, C. Dean, P. Narang, A. N. Pasupathy, D. M. Kennes, and D. N. Basov, Unconventional non-local relaxation dynamics in a twisted trilayer graphene moiré superlattice, Nat. Commun. 13, 7587 (2022).
  10. M. Van Winkle, I. M. Craig, S. Carr, M. Dandu, K. C. Bustillo, J. Ciston, C. Ophus, T. Taniguchi, K. Watanabe, A. Raja, S. M. Griffin, and D. K. Bediako, Rotational and dilational reconstruction in transition metal dichalcogenide moiré bilayers, Nat. Commun. 14, 2989 (2023).
  11. A. Uri, S. Grover, Y. Cao, J. A. Crosse, K. Bagani, D. Rodan-Legrain, Y. Myasoedov, K. Watanabe, T. Taniguchi, P. Moon, M. Koshino, P. Jarillo-Herrero, and E. Zeldov, Mapping the twist-angle disorder and Landau levels in magic-angle graphene, Nature (London) 581, 47 (2020).
  12. S. Zhao, Z. Li, X. Huang, A. Rupp, J. Göser, I. A. Vovk, S. Y. Kruchinin, K. Watanabe, T. Taniguchi, I. Bilgin, A. S. Baimuratov, and A. Högele, Excitons in mesoscopically reconstructed moiré heterostructures, Nat. Nanotechnol. 18, 572 (2023).
  13. F. Cadiz, E. Courtade, C. Robert, G. Wang, Y. Shen, H. Cai, T. Taniguchi, K. Watanabe, H. Carrere, D. Lagarde, M. Manca, T. Amand, P. Renucci, S. Tongay, X. Marie, and B. Urbaszek, Excitonic linewidth approaching the homogeneous limit in MoS2-based van der Waals heterostructures, Phys. Rev. X 7, 021026 (2017).
  14. See Supplemental Material at http://link.aps.org/supplemental/10.1103/qdq1-2yk9 for the experimental methods, the 1D reconstruction modeling, the 1D-confined exciton modeling, the quantification of uniaxial tensile strain, the control experiments with different mesa separations, the dependence of energy splitting Δxy on the 1D-wire width w, and the power dependence of 1D-confined exciton, which includes Refs. [15–34].
  15. A. A. Al-Hilli and B. L. Evans, The preparation and properties of transition metal dichalcogenide single crystals, J. Cryst. Growth 15, 93 (1972).
  16. P. Ji, S. Yang, Y. Wang, K. Li, Y. Wang, H. Suo, Y. T. Woldu, X. Wang, F. Wang, L. Zhang, and Z. Jiang, High-performance photodetector based on an interface engineering-assisted graphene/silicon Schottky junction, Microsyst. Nanoeng. 8, 9 (2022).
  17. L. A. Jauregui, A. Y. Joe, K. Pistunova, D. S. Wild, A. A. High, Y. Zhou, G. Scuri, K. De Greve, A. Sushko, C.-H. Yu, T. Taniguchi, K. Watanabe, D. J. Needleman, M. D. Lukin, H. Park, and P. Kim, Electrical control of interlayer exciton dynamics in atomically thin heterostructures, Science 366, 870 (2019).
  18. F. Ahmed, S. Heo, Z. Yang, F. Ali, C. H. Ra, H.-I. Lee, T. Taniguchi, J. Hone, B. H. Lee, and W. J. Yoo, Dielectric dispersion and high field response of multilayer hexagonal boron nitride, Adv. Funct. Mater. 28, 1804235 (2018).
  19. A. Laturia, M. L. Van de Put, and W. G. Vandenberghe, Dielectric properties of hexagonal boron nitride and transition metal dichalcogenides: From monolayer to bulk, npj 2D Mater. Appl. 2, 6 (2018).
  20. A. Rupp, J. Göser, Z. Li, I. Bilgin, A. Baimuratov, and A. Högele, Imaging lattice reconstruction in homobilayers and heterobilayers of transition metal dichalcogenides, 2D Mater. 10, 045028 (2023).
  21. M. Pendharkar, S. J. Tran, G. Zaborski, J. Finney, A. L. Sharpe, R. V. Kamat, S. S. Kalantre, M. Hocking, N. J. Bittner, K. Watanabe, T. Taniguchi, B. Pittenger, C. J. Newcomb, M. A. Kastner, A. J. Mannix, and D. Goldhaber-Gordon, Torsional force microscopy of van der Waals moirés and atomic lattices, Proc. Natl. Acad. Sci. U.S.A. 121, e2314083121 (2024).
  22. S. Carr, D. Massatt, S. B. Torrisi, P. Cazeaux, M. Luskin, and E. Kaxiras, Relaxation and domain formation in incommensurate two-dimensional heterostructures, Phys. Rev. B 98, 224102 (2018).
  23. V. V. Enaldiev, V. Zólyomi, C. Yelgel, S. J. Magorrian, and V. I. Fal’ko, Stacking domains and dislocation networks in marginally twisted bilayers of transition metal dichalcogenides, Phys. Rev. Lett. 124, 206101 (2020).
  24. L. D. Landau and E. M. Lifshitz, Theory of Elasticity: Volume 7 (Elsevier, Oxford, England, UK, 1986).
  25. Z. Li, F. Tabataba-Vakili, S. Zhao, A. Rupp, I. Bilgin, Z. Herdegen, B. März, K. Watanabe, T. Taniguchi, G. R. Schleder, A. S. Baimuratov, E. Kaxiras, K. Müller-Caspary, and A. Högele, Lattice reconstruction in MoSe2WSe2 heterobilayers synthesized by chemical vapor deposition, Nano Lett. 23, 4160 (2023).
  26. G. E. Pikus and G. L. Bir, Exchange interaction in excitons in semiconductors, Sov. Phys. JETP 33, 108 (1971).
  27. E. L. Ivchenko, Optical Spectroscopy of Semiconductor Nanostructures (Alpha Science, Harrow UK, 2005).
  28. H. Yu, G.-B. Liu, P. Gong, X. Xu, and W. Yao, Dirac cones and Dirac saddle points of bright excitons in monolayer transition metal dichalcogenides, Nat. Commun. 5, 3876 (2014).
  29. M. M. Glazov, T. Amand, X. Marie, D. Lagarde, L. Bouet, and B. Urbaszek, Exciton fine structure and spin decoherence in monolayers of transition metal dichalcogenides, Phys. Rev. B 89, 201302(R) (2014).
  30. A. I. Prazdnichnykh, M. M. Glazov, L. Ren, C. Robert, B. Urbaszek, and X. Marie, Control of the exciton valley dynamics in atomically thin semiconductors by tailoring the environment, Phys. Rev. B 103, 085302 (2021).
  31. E. Wietek, M. Florian, J. Göser, T. Taniguchi, K. Watanabe, A. Högele, M. M. Glazov, A. Steinhoff, and A. Chernikov, Nonlinear and negative effective diffusivity of interlayer excitons in moiré-free heterobilayers, Phys. Rev. Lett. 132, 016202 (2024).
  32. B. Aslan, M. Deng, and T. F. Heinz, Strain tuning of excitons in monolayer WSe2, Phys. Rev. B 98, 115308 (2018).
  33. Y. Li, T. Wang, H. Wang, Z. Li, Y. Chen, D. West, R. Sankar, R. K. Ulaganathan, F. Chou, C. Wetzel, C.-Y. Xu, S. Zhang, and S.-F. Shi, Enhanced light emission from the ridge of two-dimensional InSe flakes, Nano Lett. 18, 5078 (2018).
  34. R. Ai, X. Cui, Y. Li, and X. Zhuo, Local strain engineering of two-dimensional transition metal dichalcogenides towards quantum emitters, Nano-Micro Lett. 17, 104 (2025).
  35. Y. Dong, M.-M. Yang, M. Yoshii, S. Matsuoka, S. Kitamura, T. Hasegawa, N. Ogawa, T. Morimoto, T. Ideue, and Y. Iwasa, Giant bulk piezophotovoltaic effect in 3RMoS2, Nat. Nanotechnol. 18, 36 (2023).
  36. M. R. Rosenberger, H.-J. Chuang, M. Phillips, V. P. Oleshko, K. M. McCreary, S. V. Sivaram, C. S. Hellberg, and B. T. Jonker, Twist Angle-dependent atomic reconstruction and moiré patterns in transition metal dichalcogenide heterostructures, ACS Nano 14, 4550 (2020).
  37. T. I. Andersen, G. Scuri, A. Sushko, K. De Greve, J. Sung, Y. Zhou, D. S. Wild, R. J. Gelly, H. Heo, D. Bérubé, A. Y. Joe, L. A. Jauregui, K. Watanabe, T. Taniguchi, P. Kim, H. Park, and M. D. Lukin, Excitons in a reconstructed moiré potential in twisted WSe2/WSe2 homobilayers, Nat. Mater. 20, 480 (2021).
  38. J. S. Alden, A. W. Tsen, P. Y. Huang, R. Hovden, L. Brown, J. Park, D. A. Muller, and P. L. McEuen, Strain solitons and topological defects in bilayer graphene, Proc. Natl. Acad. Sci. U.S.A. 110, 11256 (2013).
  39. I. V. Lebedeva and A. M. Popov, Commensurate-incommensurate phase transition and a network of domain walls in bilayer graphene with a biaxially stretched layer, Phys. Rev. B 99, 195448 (2019).
  40. V. V. Enaldiev, Dislocations in twistronic heterostructures, 2D Mater. 11, 035014 (2024).
  41. M. Förg, A. S. Baimuratov, S. Yu. Kruchinin, I. A. Vovk, J. Scherzer, J. Förste, V. Funk, K. Watanabe, T. Taniguchi, and A. Högele, Moiré excitons in MoSe2WSe2 heterobilayers and heterotrilayers, Nat. Commun. 12, 1656 (2021).
  42. E. M. Alexeev, N. Mullin, P. Ares, H. Nevison-Andrews, O. Skrypka, T. Godde, A. Kozikov, L. Hague, Y. Wang, K. S. Novoselov, L. Fumagalli, J. K. Hobbs, and A. I. Tartakovskii, Emergence of highly linearly polarized interlayer exciton emission in MoSe2/WSe2 heterobilayers with transfer-induced layer corrugation, ACS Nano 14, 11110 (2020).
  43. Y. Bai, L. Zhou, J. Wang, W. Wu, L. J. McGilly, D. Halbertal, C. F. B. Lo, F. Liu, J. Ardelean, P. Rivera, N. R. Finney, X.-C. Yang, D. N. Basov, W. Yao, X. Xu, J. Hone, A. N. Pasupathy, and X.-Y. Zhu, Excitons in strain-induced one-dimensional moiré potentials at transition metal dichalcogenide heterojunctions, Nat. Mater. 19, 1068 (2020).
  44. D. Thureja, A. Imamoglu, T. Smoleński, I. Amelio, A. Popert, T. Chervy, X. Lu, S. Liu, K. Barmak, K. Watanabe, T. Taniguchi, D. J. Norris, M. Kroner, and P. A. Murthy, Electrically tunable quantum confinement of neutral excitons, Nature (London) 606, 298 (2022).
  45. P. Ils, C. Gréus, A. Forchel, V. D. Kulakovskii, N. A. Gippius, and S. G. Tikhodeev, Linear polarization of photoluminescence emission and absorption in quantum-well wire structures: Experiment and theory, Phys. Rev. B 51, 4272 (1995).
  46. L. A. Jauregui, A. Y. Joe, K. Pistunova, D. S. Wild, A. A. High, Y. Zhou, G. Scuri, K. De Greve, A. Sushko, C.-H. Yu, T. Taniguchi, K. Watanabe, D. J. Needleman, M. D. Lukin, H. Park, and P. Kim, Electrical control of interlayer exciton dynamics in atomically thin heterostructures, Science 366, 870 (2019).
  47. R. Gillen and J. Maultzsch, Interlayer excitons in MoSe2/WSe2 heterostructures from first principles, Phys. Rev. B 97, 165306 (2018).
  48. J. T. Glückert, L. Adamska, W. Schinner, M. S. Hofmann, S. K. Doorn, S. Tretiak, and A. Högele, Dipolar and charged localized excitons in carbon nanotubes, Phys. Rev. B 98, 195413 (2018).
  49. E. Barré, O. Karni, E. Liu, A. L. O’Beirne, X. Chen, H. B. Ribeiro, L. Yu, B. Kim, K. Watanabe, T. Taniguchi, K. Barmak, C. H. Lui, S. Refaely-Abramson, F. H. da Jornada, and T. F. Heinz, Optical absorption of interlayer excitons in transition-metal dichalcogenide heterostructures, Science 376, 406 (2022).
  50. P. E. Faria Junior and J. Fabian, Signatures of electric field and layer separation effects on the spin-valley physics of MoSe2/WSe2 heterobilayers: From energy bands to dipolar excitons, Nanomaterials 13, 1187 (2023).
  51. A. Weston et al., Interfacial ferroelectricity in marginally twisted 2D semiconductors, Nat. Nanotechnol. 17, 390 (2022).
  52. M. Heithoff, A. Moreno, I. Torre, M. S. G. Feuer, C. M. Purser, G. M. Andolina, G. Calajò, K. Watanabe, T. Taniguchi, D. M. Kara, P. Hays, S. A. Tongay, V. I. Fal’ko, D. Chang, M. Atatüre, A. Reserbat-Plantey, and F. H. L. Koppens, Valley-hybridized gate-tunable 1D exciton confinement in MoSe2, ACS Nano 18, 30283 (2024).
  53. P. Soubelet, Y. Tong, A. Astaburuaga Hernandez, P. Ji, K. Gallo, A. V. Stier, and J. J. Finley, Strong quantum confinement of 2D excitons in an engineered 1D potential induced by proximal ferroelectric domain walls, Nano Lett. 25, 12842 (2025).
  54. R. Ołdziejewski, A. Chiocchetta, J. Knörzer, and R. Schmidt, Excitonic Tonks-Girardeau and charge density wave phases in monolayer semiconductors, Phys. Rev. B 106, L081412 (2022).
  55. S. Zhao, Z. Li, Z. A. Iakovlev, P. Ji, T. Jiang, F. Lin, X. Huang, K. Watanabe, T. Taniguchi, M. Glazov, A. S. Baimuratov, and A. Högele, Strain-controlled atomic reconstruction and quasi-1D excitons in moiré heterostructures (2026), 10.5281/zenodo.18591599.

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation