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    Material Realization of Spinless, Covalent-Type Dirac Semimetals in Three Dimensions

    Yuki Tanaka1, Rinsuke Yamada1,*, Manabu Sato1, Noriyuki Kabeya2,3, Masaki Kondo4, Noriaki Kimura2, Masashi Tokunaga4,5, Motoaki Hirayama5, and Max Hirschberger1,5,†

    • *Contact author: ryamada@ap.t.u-tokyo.ac.jp
    • †Contact author: hirschberger@ap.t.u-tokyo.ac.jp

    Phys. Rev. Lett. 137, 096603 – Published 26 August, 2026

    DOI: https://doi.org/10.1103/pshy-l48q

    Abstract

    Realization of a three-dimensional (3D) analog of graphene has been a central challenge in topological materials science. Graphene is stabilized by covalent bonding, unlike conventional spin-orbit-type 3D Dirac semimetals (DSMs). In this study, we demonstrate the material realization of covalent-type 3D DSMs R8CoX3 stabilized by covalent bonding. We confirm the clean Dirac semimetal state in Y8CoIn3 by combined thermodynamic and transport experiments. We also realize high carrier mobility exceeding 3000  cm2/Vs even in polycrystalline samples of R8CoX3. Our research provides a material platform for exploration of Dirac electrons in three dimensions with wide chemical tunability.

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