Oxygen Isotope Fingerprints of Electron-Phonon Coupling in Films
Phys. Rev. Lett. 136, 076501 – Published 18 February, 2026
DOI: https://doi.org/10.1103/mtzb-b5ww
Abstract
Transition metals exemplify correlated electronic systems, where electron-electron () scattering often results in a quadratic temperature dependence of the electrical resistivity, . In (SVO), a material with a electronic configuration that ensures metallicity through narrow bands, a dependence has been reported. While traditionally attributed to scattering, recent studies suggest that electron-phonon (-ph) interactions may play a significant role. To unravel the influence of phonon interactions on carrier transport in SVO, we present a comparative study of the transport and optical properties of SVO films with partial substitution of ions by their heavier isotope, . Our findings reveal that substitution induces a change in the slope of at nominal fixed carrier density, highlighting the dominant contribution of -ph coupling over scattering in determining . Furthermore, it is found that the substitution softens the phonon lattice and promotes a reduction in plasma frequency and an increase in the carrier effective mass. These results indicate that the -ph coupling strength increases upon substitution. Our findings suggest that -ph interactions may surpass scattering in governing the resistivity of metallic ionic lattices.