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Orbital Magnetization of Correlated States in Twisted Bilayer Transition Metal Dichalcogenides

Xiaoyu Liu1, Chong Wang1, Haoran Chen1, Xiao-Wei Zhang1, Ting Cao1,*, and Di Xiao1,2,3,†

  • *Contact author: tingcao@uw.edu
  • Contact author: dixiao@uw.edu

Phys. Rev. Lett. 136, 166606 – Published 23 April, 2026

DOI: https://doi.org/10.1103/k46f-8m8t

Abstract

Recent observations of quantum anomalous Hall effects in moiré systems have revealed the emergence of interaction-driven ferromagnetism with significant orbital contributions. To capture this physics, we extend the modern theory of orbital magnetization to Hartree–Fock states and show that the standard expression remains valid with Hartree–Fock orbitals and Hamiltonians. Then, we benchmark our theory against the extended Kane-Mele-Hubbard model in a weak field, which yields excellent agreement with direct numerical calculations. Applying our theory to twisted MoTe2 bilayers, we find orbital magnetization of order one Bohr magneton per moiré cell with a nonmonotonic twist-angle dependence. Our work establishes a general theory of orbital magnetization in interacting moiré systems and provides quantitative guidance for interpreting recent experiments.

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