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    Control of Dipolar Dynamics by Geometrical Programming

    Jiaqi You1,2,*, John M. Doyle1,2, Zirui Liu1,2,3, Scarlett S. Yu1,2, and Avikar Periwal1,2

    • *Contact author: jiaqiyou@g.harvard.edu

    Phys. Rev. Lett. 135, 253002 – Published 18 December, 2025

    DOI: https://doi.org/10.1103/k22t-xgcy

    Abstract

    We propose and theoretically analyze methods for quantum many-body control through geometric reshaping of molecular tweezer arrays. Dynamic rearrangement during entanglement is readily available due to the extended coherence times of molecular rotational qubits. We show how motional dephasing can be suppressed and enhanced spin squeezing can be achieved in an actively rearranged short-range XY model. We also analyze in detail a specific static geometry that significantly suppresses decoherence. These general methods as applied to programmable quantum systems offer robust control modalities that are well suited to molecules.

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