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Synchronization Driven Reciprocity Breaking
Phys. Rev. Lett. 137, 033802 – Published 16 July, 2026
DOI: https://doi.org/10.1103/jln4-jg5c
Abstract
Wave transmission reciprocity is broken by exploiting the synchronization of two coupled self-oscillators. The underlying principle is that illumination from one port drives the in phase, while illumination from the other port drives the antiphase synchronization state. Because of its self-adjustment the system is operationally stable. An experimental demonstration with aeroacoustic cavities is presented. They behave as weakly nonlinear limit cycles when driven by a constant airflow, leading to self-oscillations that can couple to the surrounding waveguides via two ports. Incident waves from one port trigger antiphase synchronization, causing destructive interference and low transmission, while waves from the opposite port induce in-phase synchronization, resulting in high transmission. This directional dependence effectively breaks reciprocity, where the operational bandwidth is defined by the synchronization region and can be broader than resonance-based methods. Experimental results show robust nonreciprocal behavior with respect to parameter changes. Moreover, a modified temporal coupled mode theory is proposed, explaining the system’s nonlinear dynamics and scattering properties in a quantitative manner. This synchronization-based approach offers a new avenue for directional wave control, complementing traditional reciprocity breaking techniques and offering an intrinsic loss compensation emanating from the self-oscillation of meta-atoms.
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References (56)
- H. Nassar, B. Yousefzadeh, R. Fleury, M. Ruzzene, A. Alù, C. Daraio, A. N. Norris, G. Huang, and M. R. Haberman, Nonreciprocity in acoustic and elastic materials, Nat. Rev. Mater. 5, 667 (2020).
- C. Kittel, Interaction of spin waves and ultrasonic waves in ferromagnetic crystals, Phys. Rev. 110, 836 (1958).
- L. M. Nash, D. Kleckner, A. Read, V. Vitelli, A. M. Turner, and W. T. Irvine, Topological mechanics of gyroscopic metamaterials, Proc. Natl. Acad. Sci. U.S.A. 112, 14495 (2015).
- C. P. Wiederhold, D. L. Sounas, and A. Alù, Nonreciprocal acoustic propagation and leaky-wave radiation in a waveguide with flow, J. Acoust. Soc. Am. 146, 802 (2019).
- T. Kariyado and Y. Hatsugai, Manipulation of dirac cones in mechanical graphene, Sci. Rep. 5, 18107 (2015).
- R. Fleury, D. L. Sounas, C. F. Sieck, M. R. Haberman, and A. Alù, Sound isolation and giant linear nonreciprocity in a compact acoustic circulator, Science 343, 516 (2014).
- Y. del Valle Inclan Redondo, X. Xu, T. C. Liew, E. A. Ostrovskaya, A. Stegmaier, R. Thomale, C. Schneider, S. Dam, S. Klembt, S. Höfling et al., Non-reciprocal band structures in an exciton–polariton floquet optical lattice, Nat. Photonics 18, 548 (2024).
- M. Liu, S. Yang, W. Chen, J. Zhou, C. Zhao, and C.-W. Qiu, Nonreciprocal thermal fizeau drag radiation around asymmetric exceptional points, Phys. Rev. Lett. 135, 126902 (2025).
- Y. Hu, Y. Li, Y. Liu, B. Li, and J. Christensen, Giant elastic-wave asymmetry in a linear passive circulator, Nat. Commun. 16, 3991 (2025).
- D. L. Sounas and A. Alù, Non-reciprocal photonics based on time modulation, Nat. Photonics 11, 774 (2017).
- M. B. Zanjani, A. R. Davoyan, A. M. Mahmoud, N. Engheta, and J. R. Lukes, One-way phonon isolation in acoustic waveguides, Appl. Phys. Lett. 104, 081905 (2014).
- Z. Yu and S. Fan, Complete optical isolation created by indirect interband photonic transitions, Nat. Photonics 3, 91 (2009).
- B.-I. Popa and S. A. Cummer, Non-reciprocal and highly nonlinear active acoustic metamaterials, Nat. Commun. 5, 3398 (2014).
- R. Tirole, S. Vezzoli, D. Saxena, S. Yang, T. Raziman, E. Galiffi, S. A. Maier, J. B. Pendry, and R. Sapienza, Second harmonic generation at a time-varying interface, Nat. Commun. 15, 7752 (2024).
- A. Harwood, S. Vezzoli, T. Raziman, C. Hooper, R. Tirole, F. Wu, S. Maier, J. Pendry, S. Horsley, and R. Sapienza, Space-time optical diffraction from synthetic motion, Nat. Commun. 16, 5147 (2025).
- X. Hu, Z. Hang, J. Li, J. Zi, and C. T. Chan, Anomalous doppler effects in phononic band gaps, Phys. Rev. E 73, 015602 (2006).
- D.-W. Wang, H.-T. Zhou, M.-J. Guo, J.-X. Zhang, J. Evers, and S.-Y. Zhu, Optical diode made from a moving photonic crystal, Phys. Rev. Lett. 110, 093901 (2013).
- Y. Wang, B. Yousefzadeh, H. Chen, H. Nassar, G. Huang, and C. Daraio, Observation of nonreciprocal wave propagation in a dynamic phononic lattice, Phys. Rev. Lett. 121, 194301 (2018).
- H. Nassar, H. Chen, A. Norris, M. Haberman, and G. Huang, Non-reciprocal wave propagation in modulated elastic metamaterials, Proc. R. Soc. A 473, 20170188 (2017).
- H. Nassar, X. Xu, A. Norris, and G. Huang, Modulated phononic crystals: Non-reciprocal wave propagation and willis materials, J. Mech. Phys. Solids 101, 10 (2017).
- L. Quan, D. L. Sounas, and A. Alù, Nonreciprocal willis coupling in zero-index moving media, Phys. Rev. Lett. 123, 064301 (2019).
- Y. Liu, Z. Liang, J. Zhu, L. Xia, O. Mondain-Monval, T. Brunet, A. Alù, and J. Li, Willis metamaterial on a structured beam, Phys. Rev. X 9, 011040 (2019).
- W. Cheng and G. Hu, Acoustic skin effect with non-reciprocal willis materials, Appl. Phys. Lett. 121, 041701 (2022).
- L. Wang, J. A. I. Martínez, G. Ulliac, B. Wang, V. Laude, and M. Kadic, Non-reciprocal and non-Newtonian mechanical metamaterials, Nat. Commun. 14, 4778 (2023).
- H. Nassar, H. Chen, A. N. Norris, and G. L. Huang, Quantization of band tilting in modulated phononic crystals, Phys. Rev. B 97, 014305 (2018).
- H. Chen, L. Y. Yao, H. Nassar, and G. L. Huang, Mechanical quantum Hall effect in time-modulated elastic materials, Phys. Rev. Appl. 11, 044029 (2019).
- Z. Zhang, P. Delplace, and R. Fleury, Superior robustness of anomalous non-reciprocal topological edge states, Nature (London) 598, 293 (2021).
- Z. Zhang, P. Delplace, and R. Fleury, Anomalous topological waves in strongly amorphous scattering networks, Sci. Adv. 9, eadg3186 (2023).
- B. Liang, B. Yuan, and J.-c. Cheng, Acoustic diode: Rectification of acoustic energy flux in one-dimensional systems, Phys. Rev. Lett. 103, 104301 (2009).
- B. Liang, X. Guo, J. Tu, D. Zhang, and J. Cheng, An acoustic rectifier, Nat. Mater. 9, 989 (2010).
- M. Cotrufo, A. Cordaro, D. L. Sounas, A. Polman, and A. Alù, Passive bias-free non-reciprocal metasurfaces based on thermally nonlinear quasi-bound states in the continuum, Nat. Photonics 18, 81 (2024).
- S. Pontula, S. Vaidya, C. Roques-Carmes, S. Z. Uddin, M. Soljačić, and Y. Salamin, Non-reciprocal frequency conversion in a non-Hermitian multimode nonlinear system, Nat. Commun. 16, 7544 (2025).
- X. Guo, H. Lissek, and R. Fleury, Observation of non-reciprocal harmonic conversion in real sounds, Commun. Phys. 6, 93 (2023).
- N. Boechler, G. Theocharis, and C. Daraio, Bifurcation-based acoustic switching and rectification, Nat. Mater. 10, 665 (2011).
- C. Coulais, D. Sounas, and A. Alu, Static non-reciprocity in mechanical metamaterials, Nature (London) 542, 461 (2017).
- Z. Lu and A. N. Norris, Non-reciprocal wave transmission in a bilinear spring-mass system, J. Vib. Acoust. 142, 021006 (2020).
- T. Devaux, V. Tournat, O. Richoux, and V. Pagneux, Asymmetric acoustic propagation of wave packets via the self-demodulation effect, Phys. Rev. Lett. 115, 234301 (2015).
- J. Veenstra, O. Gamayun, X. Guo, A. Sarvi, C. V. Meinersen, and C. Coulais, Non-reciprocal topological solitons in active metamaterials, Nature (London) 627, 528 (2024).
- A. Pikovsky, M. Rosenblum, and J. Kurths, Synchronization: A Universal Concept in Nonlinear Science, Cambridge Nonlinear Science Series No. 12 (Cambridge University Press, Cambridge, England, 2001).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/jln4-jg5c for the phase of the scattering matrix elements and the TCMT derivation, which includes Ref. [41].
- A. K. Stoychev, T. Pedergnana, and N. Noiray, Synchronization under saturable nonlinearity, Chaos 34, 081102 (2024).
- A. K. Stoychev, X. Guo, U. Kuhl, and N. Noiray, Synchronization driven acoustics: The nonlinear scattering of a self-oscillating meta-atom, Phys. Rev. E 113, 044214 (2026).
- T. Pedergnana, A. Faure-Beaulieu, R. Fleury, and N. Noiray, Loss-compensated non-reciprocal scattering based on synchronization, Nat. Commun. 15, 7436 (2024).
- N. M. Krylov and N. N. Bogoliubov, Introduction to Non-Linear Mechanics (Princeton University Press, Princeton, NJ, 1950).
- S. Fan, W. Suh, and J. D. Joannopoulos, Temporal coupled-mode theory for the Fano resonance in optical resonators, J. Opt. Soc. Am. A 20, 569 (2003).
- T. Pedergnana and N. Noiray, Superradiant scattering by a limit cycle, Phys. Rev. Appl. 20, 034068 (2023).
- T. Pedergnana, J. Kölliker, L. Perniola, and N. Noiray, Cloaking obstacles using synchronization, Phys. Rev. B 111, 035427 (2025).
- Z. Zhao, C. Guo, and S. Fan, Connection of temporal coupled-mode-theory formalisms for a resonant optical system and its time-reversal conjugate, Phys. Rev. A 99, 033839 (2019).
- B. Perlman and T. Walsh, Criterion for nonreciprocal injection locking of bilateral microwave oscillators (correspondence), IEEE Trans. Microwave Theory Tech. 18, 507 (1970).
- K. Kurokawa, Injection locking of microwave solid-state oscillators, Proc. IEEE 61, 1386 (1973).
- Y. Li, W. Luo, Z. Zhao, and D. Liu, Resonant excitation-induced nonlinear mode coupling in a microcantilever resonator, Phys. Rev. Appl. 17, 054015 (2022).
- D. Navarro-Urrios, G. Arregui, M. F. Colombano, J. Jaramillo-Fernández, A. Pitanti, A. Griol, L. Mercadé, A. Martínez, and N. E. Capuj, Giant injection-locking bandwidth of a self-pulsing limit-cycle in an optomechanical cavity, Commun. Phys. 5, 330 (2022).
- M. Euler, Universal synchronization: Acoustic experiments, the phase oscillator model and mechanical analogues, Eur. J. Phys. 45, 023003 (2024).
- S. Knünz, M. Herrmann, V. Batteiger, G. Saathoff, T. W. Hänsch, K. Vahala, and T. Udem, Injection locking of a trapped-ion phonon laser, Phys. Rev. Lett. 105, 013004 (2010).
- N. T. Otterstrom, S. Gertler, Y. Zhou, E. A. Kittlaus, R. O. Behunin, M. Gehl, A. L. Starbuck, C. M. Dallo, A. T. Pomerene, D. C. Trotter, A. L. Lentine, and P. T. Rakich, Backscatter-immune injection-locked Brillouin laser in silicon, Phys. Rev. Appl. 14, 044042 (2020).
- https://polybox.ethz.ch/index.php/s/FtkH34XDSyiT5L5.