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Tracking the Photoinduced Dynamics of a Dark Excitonic State in Single-Layer via Resonant Autler-Townes Splitting
Phys. Rev. Lett. 136, 016902 – Published 6 January, 2026
DOI: https://doi.org/10.1103/j34b-hh1c
Abstract
Excitons in monolayer transition metal dichalcogenides () exhibit a Rydberg-like series of bound states, including optically dark levels. Using a three-pulse scheme, we directly track the dynamics of the dark exciton in through the Autler-Townes splitting of the bright state. The splitting, induced by a midinfrared field resonant with the transition, reveals distinct and responses to photoexcitation. This approach provides new insight into many-body effects and offers a versatile experimental framework to probe driven excitonic dynamics in quantum materials.