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Strong Magnon-Phonon Coupling in the Kagome Antiferromagnets
Phys. Rev. Lett. 135, 086703 – Published 21 August, 2025
DOI: https://doi.org/10.1103/gymx-jk1g
Abstract
Magnon-phonon hybridization in ordered materials is a crucial phenomenon with significant implications for spintronics, magnonics, and quantum materials research. We present direct experimental evidence and theoretical insights into magnon-phonon coupling in , a kagome antiferromagnet with noncollinear spin order. Using inelastic x-ray scattering and ab initio modeling, we uncover strong hybridization between planar spin fluctuations and transverse optical phonons, resulting in a large hybridization gap of . This coupling is driven by interlayer Heisenberg exchange interactions and is enhanced by the material’s symmetry and magnetic frustration. The simplicity of the structure enables clear identification of the hybridized modes, bridging theoretical predictions and experimental observations. Our findings establish as a model system for exploring magnon-phonon interactions and offer a pathway for designing materials with tunable magnetoelastic properties.