- Open Access
Subyield Dynamics in Yield-Stress Materials
Phys. Rev. Lett. 136, 164001 – Published 21 April, 2026
DOI: https://doi.org/10.1103/gkv5-9c4l
Abstract
The mechanical response of yield-stress materials below the yield point remains a subject of debate. Two of the most widely used constitutive models for these materials offer fundamentally conflicting views: one permits plastic flow at all stress levels, while the other assumes entirely recoverable viscoelasticity below yield. Using parallel superposition rheometry, we test the subyield behavior of a microgel and an emulsion. When residual slip effects are properly accounted for, both fluids exhibit bounded, periodic strain responses, offering compelling evidence that they do not flow in the studied regime. Our results indicate that the subyield regime is underpinned by nonlinear viscoelasticity and underscore the need for improved constitutive relations that capture such effects without treating yielding as a precursor for nonlinearity.
Physics Subject Headings (PhySH)
Article Text
Supplemental Material
References (30)
- N. J. Balmforth, I. A. Frigaard, and G. Ovarlez, Yielding to stress: Recent developments in viscoplastic fluid mechanics, Annu. Rev. Fluid Mech. 46, 121 (2014).
- J. Gao, C. Tang, M. A. Elsawy, A. M. Smith, A. F. Miller, and A. Saiani, Controlling self-assembling peptide hydrogel properties through network topology, Biomacromolecules 18, 826 (2017).
- M. S. Abdelgawad, S. J. Haward, A. Q. Shen, and M. E. Rosti, From yield stress to elastic instabilities: Tuning the extensional behavior of elastoviscoplastic fluids, PNAS Nexus 3, 227 (2024).
- D. Bonn, M. M. Denn, L. Berthier, T. Divoux, and S. Manneville, Yield stress materials in soft condensed matter, Rev. Mod. Phys. 89, 035005 (2017).
- E. C. Bingham, An investigation of the laws of plastic flow, Bull. Bur. Stand. 13, 309 (1916).
- H. A. Barnes, The yield stress—A review or “”—Everything flows?, J. Non-Newtonian Fluid Mech. 81, 133 (1999).
- M. Dinkgreve, J. Paredes, M. M. Denn, and D. Bonn, On different ways of measuring “the” yield stress, J. Non-Newtonian Fluid Mech. 238, 233 (2016).
- P. Coussot, Yield stress fluid flows: A review of experimental data, J. Non-Newtonian Fluid Mech. 211, 31 (2014).
- P. Saramito, A new constitutive equation for elastoviscoplastic fluid flows, J. Non-Newtonian Fluid Mech. 145, 1 (2007).
- P. Saramito, A new elastoviscoplastic model based on the Herschel–Bulkley viscoplastic model, J. Non-Newtonian Fluid Mech. 158, 154 (2009).
- K. Kamani, G. J. Donley, and S. A. Rogers, Unification of the rheological physics of yield stress fluids, Phys. Rev. Lett. 126, 218002 (2021).
- J. Griebler, G. Donley, V. Wisniewski, and S. Rogers, Strain shift measured from stress-controlled oscillatory shear: Evidence for a continuous yielding transition and new techniques to determine recovery rheology measures, J. Rheol. 68, 301 (2024).
- A. Garg, N. Bergemann, B. Smith, M. Heil, and A. Juel, Fluidisation of yield stress fluids under vibration, J. Non-Newtonian Fluid Mech. 294, 104595 (2021).
- A. Garg, N. Bergemann, B. Smith, M. Heil, and A. Juel, Fluidisation of yield stress fluids under vibration, Sci. Talks 3, 100067 (2022).
- M. T. Hossain and R. H. Ewoldt, Protorheology, J. Rheol. 68, 113 (2024).
- J. Vermant, L. Walker, P. Moldenaers, and J. Mewis, Orthogonal versus parallel superposition measurements, J. Non-Newtonian Fluid Mech. 79, 173 (1998).
- O. Korculanin, D. Hermida-Merino, H. Hirsemann, B. Struth, S. A. Rogers, and M. P. Lettinga, Anomalous structural response of nematic colloidal platelets subjected to large amplitude stress oscillations, Phys. Fluids 29, 023102 (2017).
- A. Pons, A. Amon, T. Darnige, J. Crassous, and E. Clément, Mechanical fluctuations suppress the threshold of soft-glassy solids: The secular drift scenario, Phys. Rev. E 92, 020201(R) (2015).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/gkv5-9c4l for materials preparation and rheological characterization, fitted material parameters, and complete raw and slip-corrected parallel-superposition strain histories, which includes Ref. [20].
- M. Dinkgreve, M. Fazilati, M. Denn, and D. Bonn, Carbopol: From a simple to a thixotropic yield stress fluid, J. Rheol. 62, 773 (2018).
- J. Goyon, A. Colin, G. Ovarlez, A. Ajdari, and L. Bocquet, Spatial cooperativity in soft glassy flows, Nature (London) 454, 84 (2008).
- L. Bocquet, A. Colin, and A. Ajdari, Kinetic theory of plastic flow in soft glassy materials, Phys. Rev. Lett. 103, 036001 (2009).
- G. Vleminckx, B. D. Jofore, P. Moldenaers, and C. Clasen, Effect of geometrical confinement on the flow of soft microgel particle pastes, Rheol. Acta 59, 435 (2020).
- X. Zhang, E. Lorenceau, P. Basset, T. Bourouina, F. Rouyer, J. Goyon, and P. Coussot, Wall slip of soft-jammed systems: A generic simple shear process, Phys. Rev. Lett. 119, 208004 (2017).
- D. P. Keane, E. Nikoumanesh, K. M. Kamani, S. A. Rogers, and R. Poling-Skutvik, Universal relationship between linear viscoelasticity and nonlinear yielding in soft materials, Phys. Rev. Lett. 134, 208202 (2025).
- Y. B. Fu and R. W. Ogden, Nonlinear Elasticity: Theory and Applications, London Mathematical Society Lecture Note Series (Cambridge University Press, Cambridge, England, 2001).
- F. A. Morrison, Understanding Rheology, Topics in Chemical Engineering (Oxford University Press, New York, 2001).
- A. Woodbridge, K. Amini, F. Lundell, O. Tammisola, A. Juel, R. J. Poole, and C. P. Fonte, The University of Manchester Figshare (2025), 10.48420/29376416.
- Anton Paar GmbH, MCR Evolution Series–Reference Guide, Graz, Austria (2024), accessed 19 Oct 2025.
- S. P. Meeker, R. T. Bonnecaze, and M. Cloitre, Slip and flow in soft particle pastes, Phys. Rev. Lett. 92, 198302 (2004).