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Altermagnetic and Dipolar Splitting of Magnons in FeF2

J. Sears1,*, V. O. Garlea2, D. Lederman3,4, J. M. Tranquada1, and I. A. Zaliznyak1,†

  • *Contact author: jsears@bnl.gov
  • †Contact author: zaliznyak@bnl.gov

Phys. Rev. Lett. 136, 226701 – Published 2 June, 2026

DOI: https://doi.org/10.1103/g6dt-rf8c

Abstract

FeF2 is a prototypical rutile antiferromagnet recently proposed as an altermagnet, with a magnetic symmetry that permits spin-split electronic bands and chiral magnons. Using very-high-resolution inelastic neutron scattering on a single crystal of FeF2, we show that the dominant source of magnon splitting is in fact the long-range dipolar interaction rather than altermagnetic exchange terms. At momenta where the dipolar splitting vanishes, we observe additional broadening due to altermagnetic chiral splitting and estimate this splitting to be ∼35  μeV. Polarized measurements further reveal that, where dipolar splitting is present, the chiral magnon modes become mixed and the resulting modes are predominantly linearly polarized, with at most a small chiral component. These findings highlight the significant effect of dipolar interactions on magnon chirality, particularly when altermagnetic interactions are weak.

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