Amplitude Mode in a Multigap Superconductor Investigated by Terahertz Two-Dimensional Coherent Spectroscopy
Phys. Rev. Lett. 135, 036902 – Published 16 July, 2025
DOI: https://doi.org/10.1103/g5rp-6vb1
Abstract
We have investigated the terahertz (THz) nonlinear response of the multigap superconductor , using THz two-dimensional coherent spectroscopy (THz 2DCS). With broadband THz drive fields, we identified a nonlinear response at twice the lower superconducting gap energy at the lowest temperatures. Using narrow-band THz driving pulses, we observed first (FH) and third harmonic responses. The FH intensity shows a monotonic increase with decreasing temperature when properly normalized by the driving field strength. This is distinct from the single-gap superconductor NbN, where the FH signal exhibited a resonant enhancement at temperatures when twice the gap energy was resonant with the driving photon energy, which was interpreted to originate from the superconducting amplitude mode. Our results in are consistent with a well-defined amplitude mode only at the lowest temperatures and indicate strong damping as temperature increases. This likely indicates the importance of interband coupling in and its influence on the nature of the amplitude mode and its damping.