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    Competition between Geometrical Frustration and the Kondo Effect in CePdAl Revealed by High-Resolution Magnetization

    Yusei Shimizu1,*, Shota Nakamura2, Yoichi Ikeda3, Yohei Kono4, Shunichiro Kittaka5, Toshiro Sakakibara1, and Yosikazu Isikawa6

    • *Contact author: yshimizu@issp.u-tokyo.ac.jp

    Phys. Rev. Lett. 137, 106501 – Published 4 September, 2026

    DOI: https://doi.org/10.1103/g1rn-czgb

    Abstract

    CePdAl is a heavy-fermion compound with a quasi-kagome structure, where geometrical frustration competes with the Kondo effect. Using a high-sensitivity magnetometer, we observe clear first-order metamagnetic transitions without magnetization plateaus in CePdAl at 80 mK, indicating a lifting of frustration through the suppression of the Kondo effect and spin flips of ordered moments under fields. An anomaly in the nonlinear magnetic susceptibility at 4.3 T suggests nondipolar correlations in the polarized paramagnetic state. Furthermore, we found no evidence of non-Fermi-liquid behavior in the high-field region, where the antiferromagnetic order is completely suppressed. These findings establish the essential thermodynamic constraints for understanding the field-induced spin-liquid state in CePdAl.

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