Competition between Geometrical Frustration and the Kondo Effect in CePdAl Revealed by High-Resolution Magnetization
Phys. Rev. Lett. 137, 106501 – Published 4 September, 2026
DOI: https://doi.org/10.1103/g1rn-czgb
Abstract
CePdAl is a heavy-fermion compound with a quasi-kagome structure, where geometrical frustration competes with the Kondo effect. Using a high-sensitivity magnetometer, we observe clear first-order metamagnetic transitions without magnetization plateaus in CePdAl at 80 mK, indicating a lifting of frustration through the suppression of the Kondo effect and spin flips of ordered moments under fields. An anomaly in the nonlinear magnetic susceptibility at 4.3 T suggests nondipolar correlations in the polarized paramagnetic state. Furthermore, we found no evidence of non-Fermi-liquid behavior in the high-field region, where the antiferromagnetic order is completely suppressed. These findings establish the essential thermodynamic constraints for understanding the field-induced spin-liquid state in CePdAl.
Physics Subject Headings (PhySH)
- Exotic phases of matter
- Kondo effect
- Magnetic phase transitions
- Magnetic susceptibility
- Magnetism
- Phase diagrams
- Phase transitions
- Phase transitions by order
- Quantum phase transitions
- Thermal properties
- Heavy-fermion systems
- Strongly correlated systems
- Dilution refrigerator
- Magnetization measurements
- Susceptibility measurements