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    Large Kohn Anomaly and Phonon Collapse Induced by Charge Density Wave in UPt2Si2

    Jooseop Lee1,2, Greta L. Chappell3,4, Ryan E. Baumbach3,4,*, Ayman H. Said5, and Igor A. Zaliznyak6,†

    • *Present address: Department of Physics, University of California, Santa Cruz, California 95064, USA.
    • †Contact author: zaliznyak@bnl.gov

    Phys. Rev. Lett. 135, 036705 – Published 18 July, 2025

    DOI: https://doi.org/10.1103/clg4-2zzb

    Abstract

    Using high-energy-resolution inelastic x-ray scattering, we observe anomalous softening and damping of the transverse acoustic phonon in UPt2Si2 as the system is cooled toward the charge density wave (CDW) transition temperature TCDW. The phonon exhibits a marked Kohn-type anomaly around the CDW wave vector QCDW and becomes overdamped within a finite momentum range already well above TCDW. The dispersion anomaly is consistent with potential Fermi surface nesting, which together with the extended phonon collapse indicates strong electron-phonon coupling. The transition temperature estimated from the phonon softening is markedly lower than TCDW, consistent with a primarily electronic instability rather than a phonon-driven transition. Our results establish UPt2Si2 as a prime example of a strongly correlated electron CDW system with exceptionally strong electron-phonon coupling driving phonon softening and collapse.

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