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    Discovery of Berezinskii-Kosterlitz-Thouless Correlations in the Quantum Kagome Compound Cs2Cu3SnF12

    M. S. Grbić1,*, I. Jakovac1, I. Kupčić1, H. Tanaka2,†, and M. Horvatić3

    • *Contact author: mgrbic.phy@pmf.hr
    • †Present address: Center for Entrepreneurship Education, Institute of Science Tokyo, Midori-ku, Yokohama 226-8502, Japan.

    Phys. Rev. Lett. 137, 086501 – Published 18 August, 2026

    DOI: https://doi.org/10.1103/bm42-z87g

    Abstract

    We investigate the microscopic properties of the kagome compound Cs2Cu3SnF12 using Cu63,65 nuclear quadrupolar resonance. Analysis of the local hyperfine fields below the Néel temperature TN=20  K indicates a spin structure consistent with P21/n symmetry of negative vector chirality. Measurements of the spin-lattice relaxation rate T1−1 reveal signatures of a gapless ground state and two-dimensional Berezinskii-Kosterlitz-Thouless–type correlations above TN, extending over a broad temperature range of approximately 130 K in zero magnetic field. Within the same temperature range, the observed increase in the nuclear quadrupolar resonance linewidth is consistent with short-range chiral order recently identified by neutron scattering. Our results establish Cs2Cu3SnF12 as a unique quantum kagome system exhibiting Berezinskii-Kosterlitz-Thouless behavior.

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