Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Dynamic Scaling Theory for a Field Quench near the Kasteleyn Transition in Spin Ice

Stephen Powell1 and Sukla Pal1,2

Phys. Rev. Lett. 134, 256701 – Published 23 June, 2025

DOI: https://doi.org/10.1103/b9gd-y4y6

Abstract

We present a dynamic scaling theory to describe relaxation dynamics following a magnetic-field quench near an unconventional phase transition in the magnetic material spin ice. Starting from a microscopic model, we derive an effective description for the critical dynamics in terms of the seeding and growth of string excitations, and use this to find scaling forms in terms of time, reduced temperature, and monopole fugacity. We confirm the predictions of scaling theory using Monte Carlo simulations, which also show good quantitative agreement with analytical expressions valid in the limit of low monopole density. As well as being relevant for experiments in the spin ice materials, our results open the way for the study of dynamic critical properties in a family of unconventional classical phase transitions.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (40)

  1. T. Senthil, Deconfined quantum critical points: A review, in 50 Years of the Renormalization Group (World Scientific, Singapore, 2024), Chap. 14, pp. 169–195.
  2. T. Senthil, A. Vishwanath, L. Balents, S. Sachdev, and M. P. A. Fisher, Deconfined quantum critical points, Science 303, 1490 (2004).
  3. T. Senthil, L. Balents, S. Sachdev, A. Vishwanath, and M. P. A. Fisher, Quantum criticality beyond the Landau-Ginzburg-Wilson paradigm, Phys. Rev. B 70, 144407 (2004).
  4. L. Balents, L. Bartosch, A. Burkov, S. Sachdev, and K. Sengupta, Putting competing orders in their place near the Mott transition, Phys. Rev. B 71, 144508 (2005).
  5. Z. Nussinov, C. D. Batista, B. Normand, and S. A. Trugman, High-dimensional fractionalization and spinon deconfinement in pyrochlore antiferromagnets, Phys. Rev. B 75, 094411 (2007).
  6. F. Alet, G. Misguich, V. Pasquier, R. Moessner, and J. L. Jacobsen, Unconventional continuous phase transition in a three-dimensional dimer model, Phys. Rev. Lett. 97, 030403 (2006).
  7. L. D. C. Jaubert, J. T. Chalker, P. C. W. Holdsworth, and R. Moessner, Three-dimensional Kasteleyn transition: Spin ice in a [100] field, Phys. Rev. Lett. 100, 067207 (2008).
  8. G. Chen, J. Gukelberger, S. Trebst, F. Alet, and L. Balents, Coulomb gas transitions in three-dimensional classical dimer models, Phys. Rev. B 80, 045112 (2009).
  9. S. Papanikolaou and J. J. Betouras, First-order versus unconventional phase transitions in three-dimensional dimer models, Phys. Rev. Lett. 104, 045701 (2010).
  10. N. Wilkins and S. Powell, Synchronization transition in the double dimer model on the cubic lattice, Phys. Rev. B 99, 144403 (2019).
  11. N. Wilkins and S. Powell, Interacting double dimer model on the square lattice, Phys. Rev. B 102, 174431 (2020).
  12. C. Castelnovo, R. Moessner, and S. Sondhi, Spin ice, fractionalization, and topological order, Annu. Rev. Condens. Matter Phys. 3, 35 (2012).
  13. C. L. Henley, The “Coulomb phase” in frustrated systems, Annu. Rev. Condens. Matter Phys. 1, 179 (2010).
  14. L. Balents, Spin liquids in frustrated magnets, Nature (London) 464, 199 (2010).
  15. M. J. Harris, S. T. Bramwell, D. F. McMorrow, T. Zeiske, and K. W. Godfrey, Geometrical frustration in the ferromagnetic pyrochlore Ho2Ti2O7, Phys. Rev. Lett. 79, 2554 (1997).
  16. S. T. Bramwell and M. J. Harris, The history of spin ice, J. Phys. Condens. Matter 32, 374010 (2020).
  17. C. Castelnovo, R. Moessner, and S. L. Sondhi, Magnetic monopoles in spin ice, Nature (London) 451, 42 (2008).
  18. S. Powell, Universal monopole scaling near transitions from the Coulomb phase, Phys. Rev. Lett. 109, 065701 (2012).
  19. S. Powell, Confinement of monopoles and scaling theory near unconventional critical points, Phys. Rev. B 87, 064414 (2013).
  20. P. C. Hohenberg and B. I. Halperin, Theory of dynamic critical phenomena, Rev. Mod. Phys. 49, 435 (1977).
  21. N. Goldenfeld, Lectures on Phase Transitions and the Renormalization Group, 1st ed. (CRC Press, Boca Raton, 1992).
  22. C.-W. Liu, A. Polkovnikov, and A. W. Sandvik, Dynamic scaling at classical phase transitions approached through nonequilibrium quenching, Phys. Rev. B 89, 054307 (2014).
  23. A. Jelić and L. F. Cugliandolo, Quench dynamics of the 2d XY model, J. Stat. Mech. (2011) P02032.
  24. J. Hamp, A. Chandran, R. Moessner, and C. Castelnovo, Emergent Coulombic criticality and Kibble-Zurek scaling in a topological magnet, Phys. Rev. B 92, 075142 (2015).
  25. N. Xu, C. Castelnovo, R. G. Melko, C. Chamon, and A. W. Sandvik, Dynamic scaling of topological ordering in classical systems, Phys. Rev. B 97, 024432 (2018).
  26. S. Powell and J. T. Chalker, Classical to quantum mappings for geometrically frustrated systems: Spin-ice in a [100] field, Phys. Rev. B 78, 024422 (2008).
  27. S. Mostame, C. Castelnovo, R. Moessner, and S. L. Sondhi, Tunable nonequilibrium dynamics of field quenches in spin ice, Proc. Natl. Acad. Sci. U.S.A. 111, 640 (2014).
  28. S. R. Giblin et al., Pauling entropy, metastability, and equilibrium in Dy2Ti2O7 spin ice, Phys. Rev. Lett. 121, 067202 (2018).
  29. S. Pal and S. Powell, Crossover from string to cluster dynamics following a field quench in spin ice, Phys. Rev. B 109, 094427 (2024).
  30. J. S. Gardner, M. J. P. Gingras, and J. E. Greedan, Magnetic pyrochlore oxides, Rev. Mod. Phys. 82, 53 (2010).
  31. P. W. Kasteleyn, Dimer statistics and phase transitions, J. Math. Phys. (N.Y.) 4, 287 (1963).
  32. I. A. Ryzhkin, Magnetic relaxation in rare-earth oxide pyrochlores, J. Exp. Theor. Phys. 101, 481 (2005).
  33. L. D. C. Jaubert and P. C. W. Holdsworth, Signature of magnetic monopole and Dirac string dynamics in spin ice, Nat. Phys. 5, 258 (2009).
  34. R. J. Glauber, Time-dependent statistics of the Ising model, J. Math. Phys. (N.Y.) 4, 294 (1963).
  35. M. Süzen, Effective ergodicity in single-spin-flip dynamics, Phys. Rev. E 90, 032141 (2014).
  36. The scaling functions, calculated using mean-field theory [7, 19], are Ψ±eq(v)=4v4/3ψ[±(2ln2/3)v−2/3] and Φ±eq(v)=4v2/3{ψ[±(2ln2/3)v−2/3]}2, where ψ(x) is the positive solution of ψ3−xψ−13=0.

  37. C. Paulsen, M. J. Jackson, E. Lhotel, B. Canals, D. Prabhakaran, K. Matsuhira, S. R. Giblin, and S. T. Bramwell, Far-from-equilibrium monopole dynamics in spin ice, Nat. Phys. 10, 135 (2014).
  38. A. Libál, A. del Campo, C. Nisoli, C. Reichhardt, and C. J. O. Reichhardt, Quenched dynamics of artificial colloidal spin ice, Phys. Rev. Res. 2, 033433 (2020).
  39. D. Schnoerr, G. Sanguinetti, and R. Grima, Approximation and inference methods for stochastic biochemical kinetics—a tutorial review, J. Phys. A 50, 093001 (2017).
  40. S. Powell and S. Pal, Nottingham Research Data Management Repository (2025), 10.17639/nott.7562.

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation