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Bidirectional Ultrafast Control of Charge Density Waves via Phase Competition

Honglie Ning1,*, Kyoung Hun Oh1,*, Yifan Su1,*, Zhengyan Darius Shi1, Dong Wu2, Qiaomei Liu3, B. Q. Lv1,4, Alfred Zong1,5,6, Gyeongbo Kang7 et al.

Hyeongi Choi7, Hyun-Woo J. Kim8, Seunghyeok Ha8, Jaehwon Kim8, Suchismita Sarker9, Jacob P. C. Ruff9, B. J. Kim8, N. L. Wang2,3, Todadri Senthil1, Hoyoung Jang7, and Nuh Gedik1,†

  • *These authors contributed equally to this work.
  • †Contact author: gedik@mit.edu

Phys. Rev. Lett. 135, 246504 – Published 12 December, 2025

DOI: https://doi.org/10.1103/b1vl-qlkk

Abstract

The intricate competition between coexisting charge density waves (CDWs) can lead to rich phenomena, offering unique opportunities for phase manipulation through electromagnetic stimuli. Leveraging time-resolved x-ray diffraction, we demonstrate ultrafast control of a CDW in EuTe4 upon optical excitation. At low excitation intensities, the amplitude of one of the coexisting CDW orders increases at the expense of the competing CDW, whereas at high intensities, it exhibits a nonmonotonic temporal evolution characterized by both enhancement and reduction. This transient bidirectional controllability, tunable by adjusting photoexcitation intensity, arises from the interplay between optical quenching and phase-competition-induced enhancement. Our findings, supported by phenomenological time-dependent Ginzburg-Landau theory simulations, not only clarify the relationship between the two CDWs in EuTe4, but also highlight the versatility of optical control over order parameters enabled by phase competition.

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