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    Forward Picosecond Stokes-Pulse Generation in Transient Stimulated Raman Scattering

    R. L. Carman*

    M. E. Mack†

    F. Shimizu*

    N. Bloembergen*

    • Gordon McKay Research Laboratory, Harvard University, Cambridge, Massachusetts 02138

    • United Aircraft Research Laboratories, East Hartford, Connecticut 06108

    • Gordon McKay Research Laboratory, Harvard University, Cambridge, Massachusetts 02138

    • Division of Engineering and Applied Physics, Harvard University, Cambridge, Massachusetts 02138

    • *Work supported by National Aeronautics and Space Administration Grant No. NGR 22-007-117 and by the Joint Services Electronics Program under Contract No. N00014-67-A-0298-0006.
    • †Work supported by Advanced Research Projects Agency of the Department of Defense and monitored by the Office of Naval Research under Contract No. N00014-66-C-0344.
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    Phys. Rev. Lett. 23, 1327 – Published 8 December, 1969

    DOI: https://doi.org/10.1103/PhysRevLett.23.1327

    Abstract

    The transient excitation of molecular vibrations by a picosecond laser-pulse train depends critically on the detailed shape of the exciting pulses. Stokes pulses shorter than or equal to the generating laser pulses have been observed in CCl4. Other aspects of the transient nature include the stimulation of two Stokes lines in methanol and the absence of backward Stokes radiation.

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    Phys. Rev. Lett. 23, 1327– Published 8 December, 1969
    • Received 3 October 1969

    © 1969 American Physical Society

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