Femtosecond lasers are routinely used for inducing local modification, including nanostructuring, and ultrafast laser spectroscopy in solids. However, these studies are often being performed separately making the unveiling of exciting physical properties of laser-fabricated materials out of reach. Here, we present an all-optical platform combining the fabrication of nano to micrometer size single-shot “femtosecond-laser-delamination” membranes or cavities of ferromagnetic thin films and multilayers together with their quasi in situ characterization using the Abbe-limited interferometric, ultrafast scanning photo-acoustic and magneto-plasmonic microscopies. Ferromagnetic nickel and iron cavities display high-Q acoustic resonances providing access to long-lived ultrahigh frequency coherent phonon modes in the above 100 GHz frequency range. Cavities in cobalt-gold bilayers allow for magnetically controlled surface plasmon resonance experiments in the Otto configuration, which is otherwise very difficult to implement experimentally. Quantitative experimental characterization of functional magnetic cavities, supported by the numerical modeling of all experimental data, opens an avenue to design and fabricate tunable nanoscaled femtosecond-laser-delamination architectures in thin films and multilayers.

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• Acoustics
• Irradiation effects
• Photonics
• Plasmonics
• Ultrafast phenomena
• Nanostructures