Export citation

Export citation

Choose format for download:

Download Citation

    Microscopic Theory of a Fluctuation-Induced Dynamical Crossover in Supercooled Liquids

    Corentin C. L. Laudicina1, Liesbeth M. C. Janssen1,2, and Grzegorz Szamel3

    Phys. Rev. Lett. 137, 118201 – Published 8 September, 2026

    DOI: https://doi.org/10.1103/8lw2-352q

    Abstract

    Mean-field theories of the glass transition predict a phase transition to a dynamically arrested state, yet no such transition is observed in experiments or simulations of finite-dimensional systems. We resolve this long-standing discrepancy by incorporating critical dynamical fluctuations into a microscopic mode-coupling framework. We show that these fluctuations round off the mean-field singularity and restore ergodicity at all finite densities (or temperatures) without invoking activated dynamics or facilitation. The resulting effective theory describes the order parameter as a stochastic process with self-induced, annealed disorder, determined self-consistently at the mean-field level. In the β-relaxation regime it reduces to stochastic beta-relaxation theory, thereby unifying mode-coupling and replica-based approaches beyond mean field. All parameters of the stochastic beta-relaxation theory are fixed by the static structure, enabling parameter-free predictions that extend mean-field theory into finite dimensions.

    Physics Subject Headings (PhySH)

    See Also

    Theory of β relaxation beyond mode-coupling theory: A microscopic treatment

    Corentin C. L. Laudicina, Liesbeth M. C. Janssen, and Grzegorz Szamel
    Phys. Rev. E 114, 035411 (2026)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation