Emergent Dispersive Multipolar Excitations in
Phys. Rev. Lett. 135, 256503 – Published 18 December, 2025
DOI: https://doi.org/10.1103/7k9l-j1kh
Abstract
In most condensed-matter systems, local and collective excitations remain decoupled due to their distinct energy scales. Here, we identify the coupled local-collective excitations in the triangular antiferromagnet , by combining neutron spectroscopy with a total angular momentum modeling. The low-lying crystalline electric field (CEF) doublets include a dipolar ground state forming a stripe- order and a excited state with dipole-octupole character. High-resolution spectra reveal emergent symmetry-selected dispersions where magnon branches from the ground state are replicated on higher levels but couple with the levels to form a distinct multipolar band. An applied magnetic field reconstructs the CEF wave functions and polarizes the system into a multipolar ferromagnet, further reshaping the spectra. The study demonstrates the emergent coupling of local and collective excitations driven by strong spin-orbit coupling and establishes as a platform for field-tunable multipolar excitations in frustrated magnets.