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    Emergent Dispersive Multipolar Excitations in NaErSe2

    Zheng Zhang1, Mingfang Shu2,3, Mingtai Xie1,4, Weizhen Zhuo1,4, Yanzhen Cai1,3, Christian Balz5, Jianting Ji1, Feng Jin1, Jie Ma2,* et al.

    Qingming Zhang1,4,†

    • *Contact author: jma3@sjtu.edu.cn
    • †Contact author: qmzhang@iphy.ac.cn

    Phys. Rev. Lett. 135, 256503 – Published 18 December, 2025

    DOI: https://doi.org/10.1103/7k9l-j1kh

    Abstract

    In most condensed-matter systems, local and collective excitations remain decoupled due to their distinct energy scales. Here, we identify the coupled local-collective excitations in the triangular antiferromagnet NaErSe2, by combining neutron spectroscopy with a total angular momentum modeling. The low-lying crystalline electric field (CEF) doublets include a dipolar Γ4 ground state forming a stripe-x order and a Γ5,6 excited state with dipole-octupole character. High-resolution spectra reveal emergent symmetry-selected dispersions where magnon branches from the ground state are replicated on higher Γ4 levels but couple with the Γ5,6 levels to form a distinct multipolar band. An applied magnetic field reconstructs the CEF wave functions and polarizes the system into a multipolar ferromagnet, further reshaping the spectra. The study demonstrates the emergent coupling of local and collective excitations driven by strong spin-orbit coupling and establishes NaErSe2 as a platform for field-tunable multipolar excitations in frustrated magnets.

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