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    Spontaneous Spin-Orbit Coupling Induced by Quantum Phonon Dynamics

    Xiangyu Zhang1,2, Da Wang3,4,*, and Congjun Wu2,5,6,7,†

    • 1Department of Physics, Fudan University, Shanghai 200433, China
    • 2New Cornerstone Science Laboratory, Department of Physics, School of Science, Westlake University, Hangzhou 310024, Zhejiang, China
    • 3National Laboratory of Solid State Microstructures & School of Physics, Nanjing University, Nanjing 210093, China
    • 4Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210093, China
    • 5Institute for Theoretical Sciences, Westlake University, Hangzhou 310024, Zhejiang, China
    • 6Key Laboratory for Quantum Materials of Zhejiang Province, School of Science, Westlake University, Hangzhou 310024, Zhejiang, China
    • 7Institute of Natural Sciences, Westlake Institute for Advanced Study, Hangzhou 310024, Zhejiang, China

    • *Contact author: dawang@nju.edu.cn
    • †Contact author: wucongjun@westlake.edu.cn

    Phys. Rev. Lett. 135, 026505 – Published 8 July, 2025

    DOI: https://doi.org/10.1103/7hv4-kmhd

    Abstract

    Spin-orbit coupling is a important focus of condensed matter physics as well as electron-phonon interaction. Traditionally spin-orbit coupling is regarded as a single-body effect arising from relativity, and electron-phonon interaction is often considered spin-independent. In this Letter, we bridge spin-orbit coupling and electron-phonon interaction, and propose a novel mechanism to dynamically generate spin-orbit coupling. Based on symmetry analysis, a spin-dependent electron-phonon coupling model is constructed, and is solved by sign-problem-free quantum Monte Carlo simulations. The phase diagram versus phonon frequency ω and coupling constant λ is fully investigated. The spin-orbit coupling emerges as an order in the ground state for any λ in the adiabatic limit, accompanied by a breathing mode of lattice distortion and a staggered loop spin current. This phase dominates in the entire range of ω with λ<λ∞, a critical value in the ω→∞ limit. At λ>λ∞, the emergent spin-orbit coupling is suppressed as increasing ω, and a phase transition occurs leading to charge-density-wave ordering degenerate with superconductivity. Our work opens up the possibility of hidden spin-orbit coupling in materials where it is otherwise forbidden by lattice symmetry and paves the way to explore possible materials for spintronics.

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