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    Intrinsic Dynamic Generation of Spin Polarization by Time-Varying Electric Field

    Xukun Feng1,2,*, Jin Cao3,*, Zhi-Fan Zhang2,*, Lay Kee Ang1, Shen Lai3, Hua Jiang2,4,†, Cong Xiao2,‡, and Shengyuan A. Yang5,3,§

    • *These authors contributed equally to this work.
    • †Contact author: jianghuaphy@fudan.edu.cn
    • ‡Contact author: congxiao@fudan.edu.cn
    • §Contact author: shengyuan.yang@polyu.edu.hk

    Phys. Rev. Lett. 135, 106301 – Published 3 September, 2025

    DOI: https://doi.org/10.1103/7blz-pswv

    Abstract

    Electric control of spin in insulators is desired for low-consumption and ultrafast spintronics, but the underlying mechanism remains largely unexplored. Here, we propose an intrinsic effect of dynamic spin generation driven by time-varying electric field. In the intraband response regime, it can be nicely formulated as a Berry curvature effect and leads to two phenomena that are forbidden in the dc limit: linear spin generation in nonmagnetic insulators and intrinsic Néel spin-orbit torque in PT-symmetric antiferromagnetic insulators. These phenomena are driven by the time derivative of field rather than the field itself, and have a quantum origin in the first-order dynamic anomalous spin polarizability. Combined with first-principles calculations, we predict sizable effects driven by the terahertz field in nonmagnetic monolayer Bi and in antiferromagnetic even-layer MnBi2Te4, which can be detected in experiment.

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