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    Dimensionality-Driven Anomalous Metallic State with Zero-Field Nonreciprocal Transport in Layered Ising Superconductors

    Yanwei Cui1,*, Zenglin Liu1,*, Qin Liu1,*, Junlin Xiong1,*, Yongqin Xie1, Yudi Dai1, Ji Zhou1, Lizheng Wang1, Hanyan Fang1 et al.

    Haiwen Liu2, Shi-Jun Liang1,3, Bin Cheng1,4,†, and Feng Miao1,3,‡

    • 1National Laboratory of Solid State Microstructures, Institute of Brain-Inspired Intelligence, School of Physics, Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210093, China
    • 2Center for Advanced Quantum Studies, Department of Physics, Beijing Normal University, Beijing 100875, China
    • 3Jiangsu Physical Science Research Center, Nanjing 210093, China
    • 4Institute of Interdisciplinary Physical Sciences, School of Science, Nanjing University of Science and Technology, Nanjing 210094, China

    • *These authors contributed equally to this work.
    • †Contact author: bincheng@njust.edu.cn
    • ‡Contact author: miao@nju.edu.cn

    Phys. Rev. Lett. 135, 076501 – Published 11 August, 2025

    DOI: https://doi.org/10.1103/5qvz-d3vl

    Abstract

    The anomalous metal state (AMS), observed in “failed” superconductors, provides insights into superconductivity and quantum criticality, with studies revealing unconventional quantum phases like the Bose metal. Recently, layered transition metal dichalcogenide (TMD) superconductors approaching the two-dimensional limit have garnered significant attention for the enhanced phase fluctuations and electronic correlations. Investigating AMSs in these systems, particularly in the absence of an external magnetic field, could offer valuable insights into the dimensionality-driven emergence of exotic quantum phenomena, including triplet Cooper pairing, phase fluctuation dynamics, and especially the recently discovered field-free superconducting diode effects. However, the field-free AMS has yet to be observed in TMD superconductors. Here, we report the dimensionality-tunable AMS near the superconducting quantum phase transitions in a layered TMD superconductor 2H−Ta2S3Se. In samples with thicknesses below 10 nm, we demonstrate magnetic field-driven AMS under external magnetic field, characterized by the vanishing of the Hall resistance and the presence of finite longitudinal resistance. Remarkably, an unexpected zero-field AMS emerges as the sample thickness is reduced to 3 nm. This AMS aligns well with the quantum vortex creep model and exhibits nonreciprocal transport behaviors, suggesting the onset of spontaneous time-reversal symmetry breaking accompanied by vortex motion as the system approaches the two-dimensional limit. Our findings open new avenues for exploring dimensionality-driven exotic superconducting quantum critical phases and pave the way for a deeper understanding of zero-field superconducting diode effects.

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