- Open Access
Nanoparticle Stored with an Atomic Ion in a Linear Paul Trap
Phys. Rev. Lett. 135, 213602 – Published 21 November, 2025
DOI: https://doi.org/10.1103/5lzj-f61x
Abstract
Radiofrequency (RF) traps enable highly controlled interactions between charged particles, including reactions between cold molecular ions, sympathetic cooling of one ion species with another, and quantum logic spectroscopy. However, the charge-to-mass () selectivity of RF traps limits the range of objects that can be confined simultaneously in the same trap. Here, we confine two particles—a nanoparticle and an atomic ion—in the same radiofrequency trap although their charge-to-mass ratios differ by six orders of magnitude. The confinement is enabled by a dual-frequency voltage applied to the trap electrodes. We introduce a robust loading procedure under ultrahigh vacuum and characterize the stability of both particles. It is observed that slow-field micromotion, an effect specific to the dual-field setting, plays a crucial role for ion localization. Our results lay the groundwork for controlled interactions between diverse charged particles, regardless of the difference in their charge or mass, with applications from antimatter synthesis to the generation of macroscopic quantum states of motion.
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References (39)
- R. E. March and J. F. J. Todd, Quadrupole Ion Trap Mass Spectrometry, 2nd ed. (Wiley-Interscience, Hoboken, New Jersey, 2005).
- S. Willitsch, Coulomb-crystallised molecular ions in traps: Methods, applications, prospects, Int. Rev. Phys. Chem. 31, 175 (2012).
- D. Wineland, C. Monroe, W. Itano, D. Leibfried, B. King, and D. Meekhof, Experimental issues in coherent quantum-state manipulation of trapped atomic ions, J. Res. Natl. Inst. Stand. Technol. 103, 259 (1998).
- D. Leibfried, R. Blatt, C. Monroe, and D. Wineland, Quantum dynamics of single trapped ions, Rev. Mod. Phys. 75, 281 (2003).
- C. D. Bruzewicz, J. Chiaverini, R. McConnell, and J. M. Sage, Trapped-ion quantum computing: Progress and challenges, Appl. Phys. Rev. 6, 021314 (2019).
- P. Nagornykh, J. E. Coppock, J. P. J. Murphy, and B. E. Kane, Optical and magnetic measurements of gyroscopically stabilized graphene nanoplatelets levitated in an ion trap, Phys. Rev. B 96, 035402 (2017).
- D. Budker, P. W. Graham, H. Ramani, F. Schmidt-Kaler, C. Smorra, and S. Ulmer, Millicharged dark matter detection with ion traps, PRX Quantum 3, 010330 (2022).
- W. Paul, Electromagnetic traps for charged and neutral particles, Rev. Mod. Phys. 62, 531 (1990).
- H. Dehmelt, Economic synthesis and precision spectroscopy of anti-molecular hydrogen ions in Paul trap, Phys. Scr. 1995, 423 (1995).
- D. Trypogeorgos and C. J. Foot, Cotrapping different species in ion traps using multiple radio frequencies, Phys. Rev. A 94, 023609 (2016).
- N. Leefer, K. Krimmel, W. Bertsche, D. Budker, J. Fajans, R. Folman, H. Häffner, and F. Schmidt-Kaler, Investigation of two-frequency Paul traps for antihydrogen production, Hyperfine Interact. 238, 12 (2016).
- L. Dania, D. S. Bykov, F. Goschin, M. Teller, A. Kassid, and T. E. Northup, Ultrahigh quality factor of a levitated nanomechanical oscillator, Phys. Rev. Lett. 132, 133602 (2024).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/5lzj-f61x for stability conditions in a dual-frequency Paul trap, observations of ion-loading probabilities and storage times, a calculation of the normal modes, and a discussion of prospects for sympathetic cooling and which includes Refs. [4,12,14–20].
- D. S. Bykov, L. Dania, F. Goschin, and T. E. Northup, 3D sympathetic cooling and detection of levitated nanoparticles, Optica 10, 438 (2023).
- S. Gulde, D. Rotter, P. Barton, F. Schmidt-Kaler, R. Blatt, and W. Hogervorst, Simple and efficient photo-ionization loading of ions for precision ion-trapping experiments, Appl. Phys. B 73, 861 (2001).
- D. J. Berkeland, J. D. Miller, J. C. Bergquist, W. M. Itano, and D. J. Wineland, Minimization of ion micromotion in a Paul trap, J. Appl. Phys. 83, 5025 (1998).
- J. Jin and D. A. Church, Precision lifetimes for the levels: Experiment challenges theory at the 1% level, Phys. Rev. Lett. 70, 3213 (1993).
- E. Hebestreit, M. Frimmer, R. Reimann, C. Dellago, F. Ricci, and L. Novotny, Calibration and energy measurement of optically levitated nanoparticle sensors, Rev. Sci. Instrum. 89, 033111 (2018).
- M. Harlander, R. Lechner, M. Brownnutt, R. Blatt, and W. Hänsel, Trapped-ion antennae for the transmission of quantum information, Nature (London) 471, 200 (2011).
- K. R. Brown, C. Ospelkaus, Y. Colombe, A. C. Wilson, D. Leibfried, and D. J. Wineland, Coupled quantized mechanical oscillators, Nature (London) 471, 196 (2011).
- C. Foot, D. Trypogeorgos, E. Bentine, A. Gardner, and M. Keller, Two-frequency operation of a Paul trap to optimise confinement of two species of ions, Int. J. Mass Spectrom. 430, 117 (2018).
- P. Asenbaum, S. Kuhn, S. Nimmrichter, U. Sezer, and M. Arndt, Cavity cooling of free silicon nanoparticles in high vacuum, Nat. Commun. 4, 2743 (2013).
- S. Kuhn, P. Asenbaum, A. Kosloff, M. Sclafani, B. A. Stickler, S. Nimmrichter, K. Hornberger, O. Cheshnovsky, F. Patolsky, and M. Arndt, Cavity-assisted manipulation of freely rotating silicon nanorods in high vacuum, Nano Lett. 15, 5604 (2015).
- D. S. Bykov, P. Mestres, L. Dania, L. Schmöger, and T. E. Northup, Direct loading of nanoparticles under high vacuum into a Paul trap for levitodynamical experiments, Appl. Phys. Lett. 115, 034101 (2019).
- L. Dania, D. S. Bykov, M. Knoll, P. Mestres, and T. E. Northup, Optical and electrical feedback cooling of a silica nanoparticle levitated in a Paul trap, Phys. Rev. Res. 3, 013018 (2021).
- A. N. Vamivakas, S. B. Ippolito, A. K. Swan, M. S. Ünlü, M. Dogan, E. R. Behringer, and B. B. Goldberg, Phase-sensitive detection of dipole radiation in a fiber-based high numerical aperture optical system, Opt. Lett. 32, 970 (2007).
- F. Xiong, P. Yin, T. Wu, H. Xie, R. Li, Y. Leng, Y. Li, C. Duan, X. Kong, P. Huang, and J. Du, Lens-free optical detection of thermal motion of a submillimeter sphere diamagnetically levitated in high vacuum, Phys. Rev. Appl. 16, L011003 (2021).
- S. Arnold, Determination of particle mass and charge by one electron differentials, J. Aerosol Sci. 10, 49 (1979).
- S. Schlemmer, J. Illemann, S. Wellert, and D. Gerlich, Nondestructive high-resolution and absolute mass determination of single charged particles in a three-dimensional quadrupole trap, J. Appl. Phys. 90, 5410 (2001).
- R. Hendricks, D. Grant, P. Herskind, A. Dantan, and M. Drewsen, An all-optical ion-loading technique for scalable microtrap architectures, Appl. Phys. B 88, 507 (2007).
- B. E. King, C. S. Wood, C. J. Myatt, Q. A. Turchette, D. Leibfried, W. M. Itano, C. Monroe, and D. J. Wineland, Cooling the collective motion of trapped ions to initialize a quantum register, Phys. Rev. Lett. 81, 1525 (1998).
- T. M. Hoang, Y. Ma, J. Ahn, J. Bang, F. Robicheaux, Z.-Q. Yin, and T. Li, Torsional optomechanics of a levitated nonspherical nanoparticle, Phys. Rev. Lett. 117, 123604 (2016).
- Y. Chu, P. Kharel, W. H. Renninger, L. D. Burkhart, L. Frunzio, P. T. Rakich, and R. J. Schoelkopf, Quantum acoustics with superconducting qubits, Science 358, 199 (2017).
- P. Arrangoiz-Arriola, E. A. Wollack, Z. Wang, M. Pechal, W. Jiang, T. P. McKenna, J. D. Witmer, R. Van Laer, and A. H. Safavi-Naeini, Resolving the energy levels of a nanomechanical oscillator, Nature (London) 571, 537 (2019).
- A. D. O’Connell, M. Hofheinz, M. Ansmann, R. C. Bialczak, M. Lenander, E. Lucero, M. Neeley, D. Sank, H. Wang, M. Weides, J. Wenner, J. M. Martinis, and A. N. Cleland, Quantum ground state and single-phonon control of a mechanical resonator, Nature (London) 464, 697 (2010).
- R. Manenti, A. F. Kockum, A. Patterson, T. Behrle, J. Rahamim, G. Tancredi, F. Nori, and P. J. Leek, Circuit quantum acoustodynamics with surface acoustic waves, Nat. Commun. 8, 975 (2017).
- M. Bild, M. Fadel, Y. Yang, U. von Lüpke, P. Martin, A. Bruno, and Y. Chu, Schrödinger cat states of a 16-microgram mechanical oscillator, Science 380, 274 (2023).
- Y. Chu and S. Gröblacher, A perspective on hybrid quantum opto- and electromechanical systems, Appl. Phys. Lett. 117, 150503 (2020).
- D. S. Bykov, L. Dania, F. Goschin, and T. E. Northrup, Data for Nanoparticle Stored with an Atomic Ion in a Linear Paul Trap, v2, Zenodo (2025), 10.5281/zenodo.10716186.