Highly Anisotropic Charge Dynamics and Spectral Weight Redistribution in the Trilayer Nickelate
Phys. Rev. Lett. 137, 076005 – Published 13 August, 2026
DOI: https://doi.org/10.1103/5j5t-sfnc
Abstract
We study the -plane and -axis charge dynamics of using optical spectroscopy. While a pronounced Drude profile, i.e., metallic response, is observed in the -plane optical conductivity , the -axis optical spectra exhibit semiconducting behavior. The zero-frequency extrapolation of the optical conductivity leads to a resistivity anisotropy exceeding 1000 at low temperatures, which is much larger than the values in iron-based superconductors but comparable to those in high- cuprates. The interband response is also highly anisotropic, showing salient orbital selectivity for light polarized in the plane and along the axis. The interband-transition peaks in both and are located at lower energies compared to density-functional-theory predictions, signifying considerable electronic correlations. By investigating the spectral weight transfer, we find that above the density-wave transition, Coulomb correlations have a marked impact on the charge dynamics of , whereas in the density-wave state, a gap opens with the Ni- orbital being involved.