Export citation

Export citation

Choose format for download:

Download Citation

    Highly Anisotropic Charge Dynamics and Spectral Weight Redistribution in the Trilayer Nickelate La4Ni3O10

    Zhe Liu1,*, Jie Li1,*, Deyuan Hu2,*, Bingke Ji1, Haoran Zhang1, Jiahao Hao3, Yaomin Dai1,†, Qing Li1, Mengjun Ou1 et al.

    Bing Xu4, Yi Lu1,‡, Meng Wang2,§, and Hai-Hu Wen1,∥

    • 1National Laboratory of Solid State Microstructures and Department of Physics, Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210093, China
    • 2Center for Neutron Science and Technology, Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-Sen University, Guangzhou, Guangdong 510275, China
    • 3Key Laboratory for Microstructural Material Physics of Hebei Province, School of Science, Yanshan University, Qinhuangdao 066004, China
    • 4Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, P.O. Box 603, Beijing 100190, China

    • *These authors contributed equally to this work.
    • †Contact author: ymdai@nju.edu.cn
    • ‡Contact author: yilu@nju.edu.cn
    • §Contact author: wangmeng5@mail.sysu.edu.cn
    • ∥Contact author: hhwen@nju.edu.cn

    Phys. Rev. Lett. 137, 076005 – Published 13 August, 2026

    DOI: https://doi.org/10.1103/5j5t-sfnc

    Abstract

    We study the ab-plane and c-axis charge dynamics of La4Ni3O10 using optical spectroscopy. While a pronounced Drude profile, i.e., metallic response, is observed in the ab-plane optical conductivity σ1ab(ω), the c-axis optical spectra σ1c(ω) exhibit semiconducting behavior. The zero-frequency extrapolation of the optical conductivity σ1(ω→0)≡1/ρdc leads to a resistivity anisotropy ρc/ρab exceeding 1000 at low temperatures, which is much larger than the values in iron-based superconductors but comparable to those in high-Tc cuprates. The interband response is also highly anisotropic, showing salient orbital selectivity for light polarized in the ab plane and along the c axis. The interband-transition peaks in both σ1ab(ω) and σ1c(ω) are located at lower energies compared to density-functional-theory predictions, signifying considerable electronic correlations. By investigating the spectral weight transfer, we find that above the density-wave transition, Coulomb correlations have a marked impact on the charge dynamics of La4Ni3O10, whereas in the density-wave state, a gap opens with the Ni-dz2 orbital being involved.

    Physics Subject Headings (PhySH)

    Authorization Required

    We need you to provide your credentials before accessing this content.

    Supplemental Material (Subscription Required)

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation