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Collective Magnetic Excitations in a Photoexcited Electron-Doped Cuprate Superconductor

Daniel Jost1,*, Jiarui Li1,*, Jordyn Hales2, Jonathan Sobota1, Giacomo Merzoni3,4, Leonardo Martinelli4,§, Shuhan Ding2, Ke-Jun Xu1,5,7, Justine Schlappa3 et al.

Andreas Scherz3, Robert Carley3, Benjamin E. Van Kuiken3, Teguh C. Asmara3, Le Phuong Hoang3, Laurent Mercadier3, Sergii Parchenko3, Martin Teichmann3, Patrick S. Kirchmann1, Giacomo Ghiringhelli4,6, Brian Moritz1, Zhi-Xun Shen1,7,5,8, Thomas P. Devereaux1,9,7, Yao Wang2,†, and Wei-Sheng Lee1,‡

  • *These authors contributed equally to this work.
  • †Contact author: yao.wang@emory.edu
  • ‡Contact author: leews@stanford.edu
  • §Present address: Physik-Institut, Universität Zürich, Winterthurerstrasse 190, CH-8057 Zürich, Switzerland.

Phys. Rev. Lett. 137, 096502 – Published 26 August, 2026

DOI: https://doi.org/10.1103/2h9x-8tjk

Abstract

Elucidating the microscopic behavior of cuprates under ultrafast photoexcitation offers critical insights into their highly correlated out-of-equilibrium states. Although quasiparticle dynamics have been investigated extensively, the behavior of collective magnetic excitations remains comparatively unexplored. Here, we use time-resolved resonant inelastic x-ray scattering at the Cu L3-edge to track the collective magnetic excitations (paramagnons) in an optimally electron-doped cuprate driven out-of-equilibrium by a femtosecond pump laser pulse. Upon pumping, we observed an anti-Stokes signal associated with paramagnon generation, which modifies the paramagnon dispersion near the zone center, although the bandwidth remained unchanged. Moreover, the spectral weight exhibits a momentum-dependent variation across the Brillouin zone. The light-driven boost of the paramagnon population and the resulting spectral-weight transfer could provide new leverage to manipulate the properties of cuprates.

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