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    Mechanochemical Feedback Drives Complex Inertial Dynamics in Active Solids

    Siddhartha Sarkar1,2,*, Biswarup Ash1,*, Yueyang Wu1, Nicholas Boechler3,4,†, Suraj Shankar1,‡, and Xiaoming Mao1,§

    • *These authors contributed equally to this work.
    • †Contact author: nboechler@ucsd.edu
    • ‡Contact author: surajsh@umich.edu
    • §Contact author: maox@umich.edu

    Phys. Rev. Lett. 135, 258301 – Published 16 December, 2025

    DOI: https://doi.org/10.1103/19rh-3whq

    Abstract

    Active solids combine internal active driving with elasticity to realize states with nonequilibrium mechanics and autonomous motion. They are often studied in overdamped settings, e.g., in soft materials, and the role of inertia is less explored. We construct a model of a chemically active solid that incorporates mechanochemical feedback and show that, when feedback overwhelms mechanical damping, autonomous inertial dynamics can spontaneously emerge through sustained consumption of chemical fuel. By combining numerical simulations, analysis, and dynamical systems approaches, we show how active feedback drives complex nonlinear dynamics on multiple timescales, including limit cycles and chaos. Our results suggest design principles for creating ultrafast actuators and autonomous machines from soft, chemically powered solids.

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