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Influence of the magnetic sublattices in the double perovskite LaCaNiReO6

Konstantinos Papadopoulos1, Ola Kenji Forslund1,2, Elisabetta Nocerino2, Fredrik O. L. Johansson3,4,5, Gediminas Simutis1,6, Nami Matsubara2, Gerald Morris7, Bassam Hitti7, Donald Arseneau7 et al.

Peter Svedlindh8, Marisa Medarde9, Daniel Andreica10, Jean-Christophe Orain11, Vladimir Pomjakushin12, Lars Börjesson1, Jun Sugiyama13, Martin Månsson2, and Yasmine Sassa1,*

  • 1Department of Physics, Chalmers University of Technology, SE-412 96 Göteborg, Sweden
  • 2Department of Applied Physics, KTH Royal Institute of Technology, SE-106 91 Stockholm, Sweden
  • 3Division of Molecular and Condensed Matter Physics, Uppsala University, SE-752 37 Uppsala, Sweden
  • 4Division of Applied Physical Chemistry, KTH Royal Institute of Technology, SE-100 44 Stockholm, Sweden
  • 5Sorbonne Universite, UMR CNRS 7588, Institut des Nanosciences de Paris, F-75005 Paris, France
  • 6Laboratory for Neutron and Muon Instrumentation, Paul Scherrer Institut, CH-5232 Villigen PSI, Switzerland
  • 7TRIUMF, 4004 Wesbrook Mall, Vancouver, BC, V6T 2A3, Canada
  • 8Uppsala University, Department of Materials Science and Engineering, Uppsala University, 751 03 Uppsala, Sweden
  • 9Laboratory for Multiscale Materials Experiments, Paul Scherrer Institut, CH-5232 Villigen PSI, Switzerland
  • 10Faculty of Physics, Babes-Bolyai University, 400084 Cluj-Napoca, Romania
  • 11Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland
  • 12Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland
  • 13Neutron Science and Technology Center, Comprehensive Research Organization for Science and Society (CROSS), Tokai, Ibaraki 319-1106, Japan

  • *yasmine.sassa@chalmers.se
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Phys. Rev. B 106, 214410 – Published 8 December, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.214410

Abstract

The magnetism of double perovskites is a complex phenomenon, determined from intra- or interatomic magnetic moment interactions, and strongly influenced by geometry. We take advantage of the complementary length and timescales of the muon spin rotation, relaxation, and resonance (μ+SR) microscopic technique and bulk ac/dc magnetic susceptibility measurements to study the magnetic phases of the LaCaNiReO6 double perovskite. As a result, we are able to discern and report ferrimagnetic ordering below TC=102K and the formation of different magnetic domains above TC. Between TC<T<270K, the following two magnetic environments appear, a dense spin region and a static-dilute spin region. The paramagnetic state is obtained only above T>270K. An evolution of the interaction between Ni and Re magnetic sublattices, in this geometrically frustrated fcc perovskite structure, is revealed as a function of temperature through the critical behavior and thermal evolution of microscopic and macroscopic physical quantities.

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Phys. Rev. B 106, 214410– Published 8 December, 2022
  • Received 11 April 2022
  • Revised 25 June 2022
  • Accepted 16 September 2022
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Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. Funded by Bibsam.

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