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    Observation of laser-assisted electron-impact ionization in ultrashort intense laser fields

    Takashi Hiroi1,2, Yuya Morimoto3,*, Reika Kanya1,4,5, and Kaoru Yamanouchi1,†

    • 1Department of Chemistry, School of Science, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan
    • 2International Center for Young Scientists, National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan
    • 3Friedrich-Alexander Universität Erlangen-Nürnberg, Staudtstraße 1, 91058 Erlangen, Germany
    • 4Department of Chemistry, Faculty of Science, Tokyo Metropolitan University, 1-1 Minami-Osawa, Hachioji-shi, Tokyo 192-0397, Japan
    • 5JST PRESTO, 1-1 Minami-Osawa, Hachioji-shi, Tokyo 192-0397, Japan

    • *Present address: Ultrashort Electron Beam Science RIKEN Hakubi research team, RIKEN Cluster for Pioneering Research (CPR), RIKEN Center for Advanced Photonics (RAP), 2-1 Hirosawa, Wako, Saitama 351-0198, Japan.
    • †Corresponding author: kaoru@chem.s.u-tokyo.ac.jp

    Phys. Rev. A 104, 062812 – Published 21 December, 2021

    DOI: https://doi.org/10.1103/PhysRevA.104.062812

    Abstract

    A laser-assisted (e, 2e) [LA(e, 2e)] process of Ar in an ultrashort (1.2 ps) near-infrared intense laser field, Ar+e−+hν→Ar++e−+e−, was observed by coincidence measurements of the fast electron scattered forward within the small-angle range and the slow electron emitted to the wide-angle range. The spectrum of the sum of the kinetic energies of fast and slow electrons exhibited a shoulder structure at the one-photon energy shift from the (e, 2e) peak for the Ar 3p orbital, which was unambiguously assigned to the LA(e, 2e) process with the one-photon energy gain. The determined triply differential cross section of the LA(e, 2e) process with one-photon gain from the laser field was approximately twice as large as a theoretical estimate and this enhancement was regarded as an evidence of the formation of light-dressed states of Ar.

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