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    Quantum spectroscopy with biphotons: Lyapunov-based input-output dynamics

    Sameer Dambal1,*, Ajay Ram Srimath Kandada2, and Eric R. Bittner1,†

    • 1Department of Physics, University of Houston, Houston, Texas 77204, USA
    • 2Department of Physics and Center for Functional Materials, Wake Forest University, 1834 Wake Forest Road, Winston-Salem, North Carolina 27109, USA

    • *Contact author: sadambal@central.uh.edu
    • †Contact author: ebittner@central.uh.edu

    Phys. Rev. A 112, 053715 – Published 17 November, 2025

    DOI: https://doi.org/10.1103/wgnx-l7qx

    Abstract

    We develop a Lyapunov-based framework to model the evolution of entangled biphotons interacting with cavity and material modes. Using Gaussian-preserving dynamics and Møller operators, we map input joint spectral amplitudes to experimentally measurable joint spectral intensities. Our model reproduces key features of observed spectra and reveals off-diagonal correlations arising from cavity decay, providing a scalable and tractable tool for quantum spectroscopic analysis.

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