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    Quantum-optical signatures of solid-state high-harmonic generation driven by squeezed coherent states

    Jingze Li1, Zijian Lyu1, Haodong Liu1, and Yunquan Liu1,2,3,*

    • 1State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-Optoelectronics, School of Physics, Peking University, Beijing 100871, China
    • 2Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, Shanxi 030006, China
    • 3Peking University Yangtze Delta Institute of Optoelectronics, Nantong, Jiangsu 226010, China

    • *Contact author: Yunquan.liu@pku.edu.cn

    Phys. Rev. A 112, 033507 – Published 5 September, 2025

    DOI: https://doi.org/10.1103/vmk1-qjpj

    Abstract

    Recently, the intersection of quantum optics and attosecond physics has attracted growing interest. Here, we study the quantum optical signatures of high-harmonic generation (HHG) from solid-state material driven by squeezed coherent states. We find that squeezed coherent states can either enhance or suppress the HHG yields compared to that driven by coherent light, depending on the photon bunching or antibunching characteristics of driving light. The analysis on semiclassical trajectories indicates that the amplitude fluctuation alters the recombination energy, while the phase fluctuation affects the birth and recombination time of electron-hole pairs. By calculating the Husimi Q distributions of HHG, we demonstrate that the squeezing of the two conjugate quadratures of driving light asymmetrically influence the squeezing phase of harmonics. Surprisingly, we find that even under coherent driving, the harmonics still exhibit squeezing due to the highly nonlinear response of solid-state HHG, which was overlooked previously. Numerical calculations of the Mandel parameter are performed to characterize the photon statistics of emitted HHG arising from different microscopic mechanisms. The results indicate that intraband radiation can exhibit a super-Poissonian distribution, while interband emission exhibits sub-Poissonian distribution under coherent driving.

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