Modulation of electron wave packets by scattering on time-harmonic potentials
Phys. Rev. A 114, 033117 – Published 28 September, 2026
DOI: https://doi.org/10.1103/r76m-4zsk
Abstract
The coherent interaction between free electrons and optical near-fields enables the active modulation of electron wave packets, which is a mechanism central to photon-induced near-field electron microscopy (PINEM). While existing theories effectively describe these interactions at high kinetic energies, the growing interest in low-energy ultrafast electron microscopy may demand frameworks that explicitly account for finite wave packet geometries and recoil effects. In this paper, we develop a rigorous three-dimensional (3D) quantum scattering theory for electron wave packets interacting with time-periodic short-range potentials, with optical near-field modulation serving as the primary motivation. By mapping the time-dependent dynamics into an extended Floquet space, we formally connect the modulation process to time-independent multichannel scattering. We evaluate the resulting scattering amplitudes using both an exact -matrix approach and a multichannel eikonal approximation. In the present 3D formulation, the eikonal approximation recovers PINEM-like probabilities, but now weighted by the incoming wave packet's transverse profile. For the parameters considered, the comparison between the two methodologies verifies the accuracy of the latter. As a benchmark application, we consider a spherically symmetric oscillating potential. This model demonstrates the generation of distinct energy sidebands and reveals that the modulation strength is sensitive to the transverse focusing of the incident electron pulse.
Physics Subject Headings (PhySH)
- Atomic & molecular processes in external fields
- Electron & positron scattering
- Electron beams & optics
- Light-matter interaction
- Scattering theory
- Strong electromagnetic field effects
- Ultrafast phenomena
- Spatial light modulators
- First-principles calculations
- Nonperturbative methods
- Schroedinger equation
- Semiclassical methods