Reuse & Permissions

It is not necessary to obtain permission to reuse this article or its components as it is available under the terms of the Creative Commons Attribution 4.0 International license. This license permits unrestricted use, distribution, and reproduction in any medium, provided attribution to the author(s) and the published article's title, journal citation, and DOI are maintained. Please note that some figures may have been included with permission from other third parties. It is your responsibility to obtain the proper permission from the rights holder directly for these figures.

Export citation

Export citation

Choose format for download:

Download Citation
  • Open Access

Quasiperiodic nondipole ionization dynamics in the x-ray stabilization regime

Aleksandr V. Boitsov*, Karen Z. Hatsagortsyan†, and Christoph H. Keitel

  • *Contact author: boitsov.aleksandr.9@gmail.com
  • †Contact author: k.hatsagortsyan@mpi-hd.mpg.de

Phys. Rev. A 114, 033110 – Published 16 September, 2026

DOI: https://doi.org/10.1103/qhyv-x54g

Abstract

Recent advances in strong x-ray laser techniques enable the study of nonlinear multiphoton ionization in extreme high-frequency fields. Although the stabilization regime in such fields is theoretically established, its modified properties in the nondipole regime for long laser pulses remains unknown. Here we numerically investigate the strong-field ionization of hydrogen or a hydrogenlike ion in a long XUV laser pulse in the nondipole regime. Our study of the time-dependent quantum dynamics reveals a quasiperiodic modulation of the ionization yield as a function of pulse duration. We demonstrate that the Coulomb-field-induced slow oscillation of the ionized electron wave packet during the interaction is responsible for the observed modulation of the ionization yield. Furthermore, we scrutinize the unusual photon momentum sharing between the photoelectron and the ion in this extreme regime. These effects are observable in upcoming x-ray free-electron laser facilities.

View figure in article

Physics Subject Headings (PhySH)

Article Text

References (63)

  1. W. Becker, F. Grasbon, R. Kopold, D. B. Milošević, G. G. Paulus, and H. Walther, Above-threshold ionization: From classical features to quantum effects, Adv. Atom. Mol. Opt. Phys. 48, 35 (2002).
  2. P. Agostini and L. F. DiMauro, The physics of attosecond light pulses, Rep. Prog. Phys. 67, 813 (2004).
  3. P. B. Corkum and F. Krausz, Attosecond science, Nat. Phys. 3, 381 (2007).
  4. F. Krausz and M. Ivanov, Attosecond physics, Rev. Mod. Phys. 81, 163 (2009).
  5. F. Krausz, Nobel lecture: Sub-atomic motions, Rev. Mod. Phys. 96, 030502 (2024).
  6. A. L'Huillier, Nobel lecture: The route to attosecond pulses, Rev. Mod. Phys. 96, 030503 (2024).
  7. P. Agostini, Nobel lecture: Genesis and applications of attosecond pulse trains, Rev. Mod. Phys. 96, 030501 (2024).
  8. M. Altarelli, The European X-ray free-electron laser: Toward an ultra-bright, high repetition-rate X-ray source, High Power Laser Sci. Eng. 3, e18 (2015).
  9. C. Bostedt, S. Boutet, D. M. Fritz, Z. Huang, H. J. Lee, H. T. Lemke, A. Robert, W. F. Schlotter, J. J. Turner, and G. J. Williams, Linac coherent light source: The first five years, Rev. Mod. Phys. 88, 015007 (2016).
  10. M. Yabashi, H. Tanaka, T. Tanaka, H. Tomizawa, T. Togashi, M. Nagasono, T. Ishikawa, J. R. Harries, Y. Hikosaka, A. Hishikawa, K. Nagaya, N. Saito, E. Shigemasa, K. Yamanouchi, and K. Ueda, Compact XFEL and AMO sciences: SACLA and SCSS, J. Phys. B: At. Mol. Opt. Phys. 46, 164001 (2013).
  11. J.-D. Fan, Y.-J. Tong, Y.-G. Nie, Z.-C. Gao, B. He, H. Luan, D.-H. Lu, J.-H. Zhang, D.-F. Zhang, X.-Y. Yuan, et al., First commissioning results of the coherent scattering and imaging endstation at the Shanghai soft X-ray free-electron laser facility, Nucl. Sci. Techn. 33, 114 (2022).
  12. S. Walker and A. Landsman, Above-threshold ionization with X-ray free-electron lasers, Commun. Phys. 7, 353 (2024).
  13. V. C. Reed and K. Burnett, Ionization of atoms in intense laser pulses using the Kramers-Henneberger transformation, Phys. Rev. A 42, 3152 (1990).
  14. A. Patel, N. J. Kylstra, and P. L. Knight, Effect of laser pulse shapes on the stabilization of a model atom, J. Phys. B: At. Mol. Opt. Phys. 32, 5759 (1999).
  15. M. Gavrila, Atomic stabilization in superintense laser fields, J. Phys. B: At. Mol. Opt. Phys. 35, R147 (2002).
  16. H. A. Kramers, Collected Scientific Papers (North-Holland, Amsterdam, 1956).
  17. W. C. Henneberger, Perturbation method for atoms in intense light beams, Phys. Rev. Lett. 21, 838 (1968).
  18. S. Azizi, U. Saalmann, and J. M. Rost, Zero-energy photoelectric effect, Phys. Rev. Lett. 134, 103201 (2025).
  19. D. A. Telnov and S.-I. Chu, Relativistic ionization probabilities and photoelectron distributions of hydrogenlike ions in superstrong electromagnetic fields, Phys. Rev. A 104, 023111 (2021).
  20. M. Protopapas, C. H. Keitel, and P. L. Knight, Relativistic mass shift effects in adiabatic intense laser field stabilization of atoms, J. Phys. B: At. Mol. Opt. Phys. 29, L591 (1996).
  21. L. N. Gaier and C. H. Keitel, Relativistic classical Monte Carlo simulations of stabilization of hydrogenlike ions in intense laser pulses, Phys. Rev. A 65, 023406 (2002).
  22. A. Staudt and C. H. Keitel, Stabilization of helium in intense high-frequency laser pulses beyond the dipole approximation, J. Phys. B: At. Mol. Opt. Phys. 36, L203 (2003).
  23. M. Protopapas, C. H. Keitel, and P. L. Knight, Atomic physics with super-high intensity lasers, Rep. Prog. Phys. 60, 389 (1997).
  24. C. H. Keitel and P. L. Knight, Monte Carlo classical simulations of ionization and harmonic generation in the relativistic domain, Phys. Rev. A 51, 1420 (1995).
  25. A. Di Piazza, C. Müller, K. Z. Hatsagortsyan, and C. H. Keitel, Extremely high-intensity laser interactions with fundamental quantum systems, Rev. Mod. Phys. 84, 1177 (2012).
  26. Linac Coherent Light Source (LCLS) in Stanford, parameters, https://lcls.slac.stanford.edu/machine/parameters.
  27. FLASH, the Free-Electron LASer in Hamburg, parameters, https://photon-science.desy.de/facilities/flash/index_eng.html.
  28. S. Dziarzhytski, N. Gerasimova, R. Goderich, T. Mey, R. Reininger, M. Rübhausen, F. Siewert, H. Weigelta, and G. Brennera, Microfocusing at the PG1 beamline at FLASH, J. Synchr. Rad. 23, 123 (2016).
  29. M. Vassholz, H. P. Hoeppe, J. Hagemann, J. M. Rosselló, M. Osterhoff, R. Mettin, T. Kurz, A. Schropp, F. Seiboth, C. G. Schroer, et al., Pump-probe X-ray holographic imaging of laser-induced cavitation bubbles with femtosecond FEL pulses, Nat. Commun. 12, 3468 (2021).
  30. Y. Tong, J. Fan, Y. Nie, Z. Guo, Z. Gao, X. Yuan, B. He, J. Chen, D. Zhang, H. Luan, J. Zhang, D. Lu, M. Xie, P. Cheng, C. Feng, T. Liu, H. Deng, B. Liu, Z. Liu, and H. Jiang, Kirkpatrick-Baez mirrors commissioning for coherent scattering and imaging endstation at SXFEL, Front. Phys. 10, 977957 (2022).
  31. M. Dondera and H. Bachau, Exploring above-threshold ionization of hydrogen in an intense X-ray laser field through nonperturbative calculations, Phys. Rev. A 85, 013423 (2012).
  32. M. Klaiber, K. Z. Hatsagortsyan, and C. H. Keitel, Above-threshold ionization beyond the dipole approximation, Phys. Rev. A 71, 033408 (2005).
  33. M. Klaiber, K. Z. Hatsagortsyan, and C. H. Keitel, Relativistic ionization rescattering with tailored laser pulses, Phys. Rev. A 74, 051803(R) (2006).
  34. M. Førre, J. P. Hansen, L. Kocbach, S. Selstø, and L. B. Madsen, Nondipole ionization dynamics of atoms in superintense high-frequency attosecond pulses, Phys. Rev. Lett. 97, 043601 (2006).
  35. Z. Zhou and S.-I. Chu, Multiphoton above-threshold ionization in superintense free-electron X-ray laser fields: Beyond the dipole approximation, Phys. Rev. A 87, 023407 (2013).
  36. A. Ludwig, J. Maurer, B. W. Mayer, C. R. Phillips, L. Gallmann, and U. Keller, Breakdown of the dipole approximation in strong-field ionization, Phys. Rev. Lett. 113, 243001 (2014).
  37. I. A. Ivanov, Spin-flip processes and nondipole effects in above-threshold ionization of hydrogen in ultrastrong laser fields, Phys. Rev. A 96, 013419 (2017).
  38. A. Sommerfeld and G. Schur, Über den Photoeffekt in der K-Schale der Atome, insbesondere über die Voreilung der Photoelektronen, Ann. Phys. 396, 409 (1930).
  39. M. J. Seaton, Momentum transfer in photo-ionization processes, J. Phys. B: At. Mol. Opt. Phys. 28, 3185 (1995).
  40. C. T. L. Smeenk, L. Arissian, B. Zhou, A. Mysyrowicz, D. M. Villeneuve, A. Staudte, and P. B. Corkum, Partitioning of the linear photon momentum in multiphoton ionization, Phys. Rev. Lett. 106, 193002 (2011).
  41. M. Klaiber, E. Yakaboylu, H. Bauke, K. Z. Hatsagortsyan, and C. H. Keitel, Under-the-barrier dynamics in laser-induced relativistic tunneling, Phys. Rev. Lett. 110, 153004 (2013).
  42. S. Chelkowski, A. D. Bandrauk, and P. B. Corkum, Photon momentum sharing between an electron and an ion in photoionization: From one-photon (photoelectric effect) to multiphoton absorption, Phys. Rev. Lett. 113, 263005 (2014).
  43. D. Cricchio, E. Fiordilino, and K. Z. Hatsagortsyan, Momentum partition between constituents of exotic atoms during laser-induced tunneling ionization, Phys. Rev. A 92, 023408 (2015).
  44. S. Chelkowski, A. D. Bandrauk, and P. B. Corkum, Photon-momentum transfer in multiphoton ionization and in time-resolved holography with photoelectrons, Phys. Rev. A 92, 051401(R) (2015).
  45. A. Hartung, S. Eckart, S. Brennecke, J. Rist, D. Trabert, K. Fehre, M. Richter, H. Sann, S. Zeller, K. Henrichs, et al., Magnetic fields alter strong-field ionization, Nat. Phys. 15, 1222 (2019).
  46. P.-L. He, M. Klaiber, K. Z. Hatsagortsyan, and C. H. Keitel, Nondipole Coulomb sub-barrier ionization dynamics and photon momentum sharing, Phys. Rev. A 105, L031102 (2022).
  47. X. Mao, H. Ni, K. Lin, P.-L. He, H. Liang, S. Eckart, F. He, K. Ueda, R. Dörner, and J. Wu, Photon momentum transfer and partitioning: From one to many, Nat. Commun. 16, 5977 (2025).
  48. A. Tasnim Aynul, L. C. Rodriguez, and C. F. d. M. Faria, Quantum beating and cyclic structures in the phase-space dynamics of the Kramers-Henneberger atom, Phys. Rev. A 111, 043102 (2025).
  49. K. Toyota, O. I. Tolstikhin, T. Morishita, and S. Watanabe, Siegert-state expansion in the Kramers-Henneberger frame: Interference substructure of above-threshold ionization peaks in the stabilization regime, Phys. Rev. A 76, 043418 (2007).
  50. K. Toyota, O. I. Tolstikhin, T. Morishita, and S. Watanabe, Interference substructure of above-threshold ionization peaks in the stabilization regime, Phys. Rev. A 78, 033432 (2008).
  51. P. V. Demekhin and L. S. Cederbaum, Dynamic interference of photoelectrons produced by high-frequency laser pulses, Phys. Rev. Lett. 108, 253001 (2012).
  52. W.-C. Jiang and J. Burgdörfer, Dynamic interference as signature of atomic stabilization, Opt. Express 26, 19921 (2018).
  53. M.-X. Wang, H. Liang, X.-R. Xiao, S.-G. Chen, W.-C. Jiang, and L.-Y. Peng, Nondipole effects in atomic dynamic interference, Phys. Rev. A 98, 023412 (2018).
  54. L. Geng, H. Liang, K. Krajewska, L.-Y. Peng, and Q. Gong, Laser-induced electron Fresnel diffraction by XUV pulses at extreme intensity, Phys. Rev. A 104, L021102 (2021).
  55. A. J. Silenko, Foldy-Wouthyusen transformation and semiclassical limit for relativistic particles in strong external fields, Phys. Rev. A 77, 012116 (2008).
  56. A. Y. Silenko, Comparative analysis of direct and “step-by-step” Foldy-Wouthuysen transformation methods, Theor. Math. Phys. 176, 987 (2013).
  57. A. J. Silenko, General method of the relativistic Foldy-Wouthuysen transformation and proof of validity of the Foldy-Wouthuysen Hamiltonian, Phys. Rev. A 91, 022103 (2015).
  58. A. V. Boitsov, K. Z. Hatsagortsyan, and C. H. Keitel, Scaling method for the numerical solution of the strong-field ionization problem in the relativistic regime, Comput. Phys. Commun. 310, 109511 (2025).
  59. L. B. Madsen and P. Lambropoulos, Scaling of hydrogenic atoms and ions interacting with laser fields: Positronium in a laser field, Phys. Rev. A 59, 4574 (1999).
  60. Y. I. Salamin and F. H. M. Faisal, Harmonic generation by superintense light scattering from relativistic electrons, Phys. Rev. A 54, 4383 (1996).
  61. L. Young, E. P. Kanter, B. K. Y. Li, A. M. March, S. T. Pratt, R. Santra, S. H. Southworth, N. Rohringer, L. F. DiMauro, G. Doumy, C. A. Roedig, N. Berrah, L. Fang, M. Hoener, P. H. Bucksbaum, J. P. Cryan, S. Ghimire, J. M. Glownia, D. A. Reis, J. D. Bozek, et al., Femtosecond electronic response of atoms to ultra-intense X-rays, Nature (London) 466, 56 (2010).
  62. A. Rudenko, L. Inhester, K. Hanasaki, X. Li, S. J. Robatjazi, B. Erk, R. Boll, K. Toyota, Y. Hao, O. Vendrell, C. Bomme, E. Savelyev, B. Rudek, L. Foucar, S. H. Southworth, C. S. Lehmann, B. Kraessig, T. Marchenko, M. Simon, K. Ueda, et al., Femtosecond response of polyatomic molecules to ultra-intense hard X-rays, Nature (London) 546, 129 (2017).
  63.  A. Boitsov, Quasiperiodic nondipole ionization dynamics in the x-ray stabilization regime, https://github.com/arboec/ionization_2D.

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation