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Second-order correlations in directed emissions in sodium atoms

Ara Tonoyan

Sushree Subhadarshinee Sahoo

Anahit Gogyan*

Oleg Tretiak and Razmik Aramyan

Alexander Akulshin

Dmitry Budker

  • *Contact author: agogyan@gmail.com

Phys. Rev. A 113, 063710 – Published 5 June, 2026

DOI: https://doi.org/10.1103/q1s4-njnb

Abstract

We report second-order intensity correlations g(2)(τ) of directional midinfrared emissions from sodium vapor under bichromatic continuous-wave excitation. Directional emission at 2.34µm in the forward direction and at 2.21µm in both forward and backward directions exhibits g(2)(0) values that exceed unity yet remain well below the thermal limit of 2, indicating subthermal photon bunching characteristics of a multimode collectively driven process rather than purely independent amplified spontaneous emission. Cross-correlation measurements reveal that the counterpropagating 2.21−µm beams are positively correlated, demonstrating dynamic coupling between the two emission channels. Persistent oscillations in g(2)(τ), observed across a broad range of pump powers, shift systematically to higher frequencies with increasing excitation power, consistent with ac Stark shifts of hyperfine sublevels. Together, these observations establish that the emission arises from a phase-matched, continuous-wave collective process combining features of mirrorless lasing and amplified spontaneous emission, with long-range dipole coherence and velocity-selective coupling governing the photon statistics and the forward-backward emission symmetry. The experiment uses a 10-cm buffer-gas-free sodium vapor cell under bichromatic excitation at 589.2 and 569.0 nm; the emitted midinfrared light is detected in a Hanbury Brown–Twiss configuration. The demonstrated backward emission is of particular interest for applications in laser guide star generation and mesospheric remote sensing, where understanding the statistical properties of the emitted light is essential for optimizing sodium-based light sources.

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References (49)

  1. D. C. Hanna, M. A. Yuratich, and D. Cotter, Nonlinear Optics of Free Atoms and Molecules (Springer, New York, 1979).
  2. D. Budker, W. Gawlik, D. F. Kimball, S. M. Rochester, V. V. Yashchuk, and A. Weis, Resonant nonlinear magneto-optical effects in atoms, Rev. Mod. Phys. 74, 1153 (2002).
  3. G. A. Pitz and M. D. Anderson, Recent advances in optically pumped alkali lasers, Appl. Phys. Rev. 4, 041101 (2017).
  4. P. P. Sorokin, N. S. Shiren, J. R. Lankard, E. C. Hammond, and T. G. Kazyaka, Stimulated electronic Raman scattering, Appl. Phys. Lett. 10, 44 (1967).
  5. C.-S. Wang, Theory of stimulated Raman scattering, Phys. Rev. 182, 482 (1969).
  6. R. W. Boyd, M. S. Malcuit, D. J. Gauthier, and K. Rząewski, Competition between amplified spontaneous emission and the four-wave-mixing process, Phys. Rev. A 35, 1648 (1987).
  7. D. Grischkowsky, J. Lankard, and P. Sorokin, An atomic Rydberg state 16−µ laser, IEEE J. Quantum Electron. 13, 392 (1977).
  8. Y. Sebbag, Y. Barash, and U. Levy, Generation of coherent mid-IR light by parametric four-wave mixing in alkali vapor, Opt. Lett. 44, 971 (2019).
  9. P. Londero, V. Venkataraman, A. R. Bhagwat, A. D. Slepkov, and A. L. Gaeta, Ultralow-power four-wave mixing with Rb in a hollow-core photonic band-gap fiber, Phys. Rev. Lett. 103, 043602 (2009).
  10. B. V. Zhdanov, M. K. Shaffer, and R. J. Knize, Diode pumped Alkali lasers: History, current state and perspectives, in CLEO/Europe and EQEC 2011 Conference Digest, OSA Technical Digest (CD) (Optica Publishing Group, 2011), paper CA1_2.
  11. A. V. Andreev, V. I. Emel'yanov, and Y. A. Il'inskii, Cooperative Effects in Optics: Superradiance and Phase Transitions (Institute of Physics, University of Reading, Berkshire, 1993).
  12. H. Cao, Lasing in random media, Waves Random Media 13, R1 (2003).
  13. S. Dubey, G. A. Kazakov, B. Heizenreder, S. Zhou, S. Bennetts, S. A. Schäffer, A. Sitaram, and F. Schreck (MoSaiQC Collaboration), Modeling of a continuous superradiant laser on the sub-MHz 1s0→3p0 transition in neutral strontium-88, Phys. Rev. Res. 7, 013292 (2025).
  14. Z. Zhang, F. Zhang, B. Xu, H. Xie, B. Fu, X. Lu, N. Zhang, S. Yu, J. Yao, Y. Cheng, and Z. Xu, High-sensitivity gas detection with air-lasing-assisted coherent Raman spectroscopy, Ultrafast Sci. 2022, 9761458 (2022).
  15. K.-M. C. Fu, G. Z. Iwata, A. Wickenbrock, and D. Budker, Sensitive magnetometry in challenging environments, AVS Quantum Sci. 2, 044702 (2020),.
  16. A. M. Akulshin, D. Budker, F. Pedreros Bustos, T. Dang, E. Klinger, S. M. Rochester, A. Wickenbrock, and R. Zhang, Remote detection optical magnetometry, Phys. Rep. 1106, 1 (2025), remote Detection Optical Magnetometry.
  17. S. Jacobs, G. Gould, and P. Rabinowitz, Coherent light amplification in optically pumped Cs vapor, Phys. Rev. Lett. 7, 415 (1961).
  18. P. P. Sorokin and J. R. Lankard, Infrared lasers resulting from photodissociation of Cs2 and Rb2, J. Chem. Phys. 51, 2929 (1969),.
  19. A. Sharma, N. D. Bhaskar, Y. Q. Lu, and W. Happer, Continuous‐wave mirrorless lasing in optically pumped atomic Cs and Rb vapors, Appl. Phys. Lett. 39, 209 (1981).
  20. A. Akulshin, D. Budker, and R. McLean, Directional infrared emission resulting from cascade population inversion and four-wave mixing in Rb vapor, Opt. Lett. 39, 845 (2014).
  21. A. M. Akulshin, F. P. Bustos, and D. Budker, Continuous-wave mirrorless lasing at 2.21 µm in sodium vapors, Opt. Lett. 43, 5279 (2018).
  22. D. Antypas, O. Tretiak, D. Budker, and A. Akulshin, Polychromatic, continuous-wave mirrorless lasing from monochromatic pumping of cesium vapor, Opt. Lett. 44, 3657 (2019).
  23. L. Allen and G. I. Peters, Amplified spontaneous emission and external signal amplification in an inverted medium, Phys. Rev. A 8, 2031 (1973).
  24. D. Kolbe, M. Scheid, A. Koglbauer, and J. Walz, Continuous-wave spontaneous lasing in mercury pumped by resonant two-photon absorption, Opt. Lett. 35, 2690 (2010).
  25. A. Ramaswamy, J. Chathanathil, D. Kanta, E. Klinger, A. Papoyan, S. Shmavonyan, A. Khanbekyan, A. Wickenbrock, D. Budker, and S. A. Malinovskaya, Mirrorless lasing: A theoretical perspective, Opt. Mem. Neural Networks 32, S443 (2023).
  26. A. Ramaswamy, D. Budker, S. Rochester, A. Papoyan, S. Shmavonyan, H. Parashar, V. V. Malinovsky, and S. A. Malinovskaya, Degenerate mirrorless lasing in thermal alkali vapors, Phys. Rev. A 113, 043733 (2026).
  27. A. Bychek, R. Holzinger, and H. Ritsch, Nanoscale mirrorless superradiant lasing, Phys. Rev. Lett. 135, 143601 (2025).
  28. R. Loudon, The Quantum Theory of Light, 2nd ed. (Clarendon, Oxford, 1983).
  29. R. H. Brown and R. Q. Twiss, Correlation between photons in two coherent beams of light, Nature (London) 177, 27 (1956).
  30. R. J. Glauber, The quantum theory of optical coherence, Phys. Rev. 130, 2529 (1963).
  31. Y. S. Ihn, K.-K. Park, Y. Kim, Y.-T. Chough, and Y.-H. Kim, Intensity correlation in frequency upconversion via four-wave mixing in rubidium vapor, J. Opt. Soc. Am. B 34, 2352 (2017).
  32. J. Wiersig, C. Gies, F. Jahnke, M. Aßmann, T. Berstermann, M. Bayer, C. Kistner, S. Reitzenstein, C. Schneider, S. Höfling, A. Forchel, C. Kruse, J. Kalden, and D. Hommel, Direct observation of correlations between individual photon emission events of a microcavity laser, Nature (London) 460, 245 (2009).
  33. T. Wang, G. P. Puccioni, and G. L. Lippi, Dynamical buildup of lasing in mesoscale devices, Sci. Rep. 5, 15858 (2015).
  34. A. M. Akulshin, N. Rahaman, S. A. Suslov, D. Budker, and R. J. McLean, Spiking dynamics of frequency upconverted field generated in continuous-wave excited rubidium vapors, J. Opt. Soc. Am. B 37, 2430 (2020).
  35. A. Akulshin, F. P. Bustos, and D. Budker, Intensity-correlated spiking of infrared and ultraviolet emission from sodium vapors, Opt. Lett. 46, 2131 (2021).
  36. A. A. C. de Almeida, A. S. Alvarez, N. R. de Melo, M. R. L. da Motta, M. P. M. de Souza, and S. S. Vianna, Intensity correlations in transmission and four-wave-mixing signals intermediated by hot rubidium atoms, Phys. Rev. A 111, 043518 (2025).
  37. A. M. Akulshin, F. P. Bustos, N. Rahaman, and D. Budker, Origin and properties of polychromatic directional emission from sodium atoms, J. Opt. Soc. Am. B 40, 3276 (2023).
  38. A. M. Akulshin, A. A. Orel, and R. J. McLean, Collimated blue light enhancement in velocity-selective pumped Rb vapour, J. Phys. B 45, 015401 (2012).
  39. J. Mika, L. Podhora, L. Lachman, P. Obšil, J. Hloušek, M. Ježek, R. Filip, and L. Slodička, Generation of ideal thermal light in warm atomic vapor, New J. Phys. 20, 093002 (2018).
  40. J. W. Goodman, Statistical Optics, 2nd ed. (Wiley, New York, 2015).
  41. W. R. Garrett, M. A. Moore, R. C. Hart, M. G. Payne, and R. Wunderlich, Suppression effects in stimulated hyper-Raman emissions and parametric four-wave mixing in sodium vapor, Phys. Rev. A 45, 6687 (1992).
  42. M. A. Moore, W. Garrett, and M. Payne, Suppression of electronic hyper-Raman emission by four-wave mixing interference, Opt. Commun. 68, 310 (1988).
  43. M. P. M. de Souza, A. A. C. de Almeida, and S. S. Vianna, Dynamic Stark shift in Doppler-broadened four-wave mixing, Phys. Rev. A 105, 053128 (2022).
  44. G. Ferioli, I. Ferrier-Barbut, and A. Browaeys, Emergence of second-order coherence in the superradiant emission from a free-space atomic ensemble, Phys. Rev. Lett. 134, 153602 (2025).
  45. J. Schmitt, T. Damm, D. Dung, F. Vewinger, J. Klaers, and M. Weitz, Observation of grand-canonical number statistics in a photon Bose-Einstein condensate, Phys. Rev. Lett. 112, 030401 (2014).
  46. NIST Atomic Spectra Database, Sodium (Na I) transition data, https://www1.udel.edu/atom/transition?element=Na1, accessed 31 Jan 2026.
  47. E. Arimondo, M. Inguscio, and P. Violino, Experimental determinations of the hyperfine structure in the alkali atoms, Rev. Mod. Phys. 49, 31 (1977).
  48. F. Biraben and K. Beroff, Hyperfine interaction in the 4D32 and the 4D52 levels of sodium, Phys. Lett. A 65, 209 (1978).
  49. B. Burghardt, M. Dubke, W. Jitschin, and G. Meisel, Sub-natural linewidth laser spectroscopy of Doppler-free two-photon resonances, Phys. Lett. A 69, 93 (1978).

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