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    Relativistic spin-flip effect in the attoclock

    I. A. Ivanov*, A. S. Kheifets†, and A. S. Landsman‡

    • *Contact author: Igor.Ivanov@anu.edu.au
    • †Contact author: A.Kheifets@anu.edu.au
    • ‡Contact author: landsman.7@osu.edu

    Phys. Rev. A 112, 023102 – Published 1 August, 2025

    DOI: https://doi.org/10.1103/pfxy-2j96

    Abstract

    We study the effect of spin flip on tunneling ionization in the attoclock settings. Our study is based on a fully relativistic approach in which we seek a numerical solution of the time-dependent Dirac equation. We find that spin flip during strong field ionization significantly increases the attoclock offset angle, indicating longer tunneling delay relative to electrons with no spin flip. To interpret our numerical findings, we conduct additional modeling within the perturbative Breit-Pauli approach, which allows us to elucidate the role of different relativistic mechanisms. We show that the spin-orbit interaction is mainly responsible for the spin flip, rather than interaction with the magnetic component of the laser field. We further discuss the dynamic mechanisms of the spin-flip effect, suggesting that it takes place while the electron is still bound. Our findings indicate that the attoclock can be used to investigate electron spin-flip dynamics during the tunnel ionization process.

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