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  • Open Access

Magnetic atoms with a large electric dipole moment

J. Seifert, S. C. Wright, B. G. Sartakov, G. Valtolina*, and G. Meijer†

  • *Contact author: valtolina@fhi-berlin.mpg.de
  • †Contact author: meijer@fhi-berlin.mpg.de

Phys. Rev. A 114, L040801 – Published 15 October, 2026

DOI: https://doi.org/10.1103/mtyy-l197

Abstract

We experimentally show that an electric dipole moment of more than 1 Debye can be induced in the dysprosium (Dy) atom, in a long-lived state that is about 17513cm−1 above the ground state. This metastable state is part of a strongly coupled opposite-parity doublet. Using optically detected microwave spectroscopy in an atomic beam, we determine the approximately 1.12cm−1 doublet spacing for the five stable bosonic isotopes of Dy with kilohertz-level accuracy. From the shift of the microwave transition frequency in low electric fields (below 150 V/cm) and from optical spectra in high electric fields (up to 150 kV/cm), a reduced transition dipole moment of 7.65 ± 0.05 Debye between the doublet states is extracted. In high electric fields the doublet interacts with a third state at 17727cm−1 that connects to the ground state via an electric-dipole transition. The three-state Stark interaction enables preparation of Dy atoms in the metastable state via single-photon excitation from the ground state. Our work experimentally validates predicted characteristics of the opposite-parity doublet and provides an effective route to the first doubly polar quantum gas of atoms.

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