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    Wavelength-dependent interband contributions to high-order harmonics in MgO crystals

    Wenli Jiang1,2,3,4, Yue Qiao3, Shicheng Jiang5,*, Yong Zhou6,†, Yujun Yang2,4,‡, and Jigen Chen1,§

    • *Contact author: scjiang@lps.ecnu.edu.cn
    • †Contact author: Zhouy5077@tzzxyy.com
    • ‡Contact author: yangyj@jlu.edu.cn
    • §Contact author: kiddchen@126.com

    Phys. Rev. A 112, 023511 – Published 19 August, 2025

    DOI: https://doi.org/10.1103/jr88-1k17

    Abstract

    By numerically solving semiconductor Bloch equations under the three-band model, we investigate the high-order harmonic emission of bulk MgO crystals irradiated by linearly polarized laser pulses. Our results reveal that as the laser wavelength increases, interband polarization dominates over intraband current near the minimum band gap (7.8 eV) in the 〈001〉 orientation, with contributions shifting toward lower-energy regions. This shift arises from enhanced electron density accumulation at the Brillouin zone boundary and increased interband harmonics between conduction bands. The findings highlight the critical role of laser wavelength in shaping harmonic contributions and deepen our understanding of high-order harmonic generation in crystalline materials.

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