Only a few states in high-dimensional systems can be identified as (un)steerable using existing theoretical or experimental methods. We utilize semidefinite programming (SDP) to construct a dataset for steerability detection in qutrit-qutrit systems. For the full-information feature $F_1$, artificial neural networks achieve high classification accuracy and generalization, and perform better than the support vector machine. As feature engineering plays a pivotal role, we introduce a steering ellipsoidlike feature, $F_2$, which significantly enhances the performance of each of our models. To address quantum steering detection in isotropic states, partially entangled states, and random states, we explore, respectively, the most tailored feature and classifier. Given that the SDP method provides only a sufficient condition for steerability detection, we establish the first rigorously constructed, accurately labeled dataset based on theoretical foundations. This dataset enables models to exhibit outstanding accuracy and generalization capabilities, independent of the choice of features. As applications, we investigate the steerability boundaries of isotropic states and partially entangled states, discover new steerable states, and determine their parameter ranges. This work not only advances the application of machine learning for probing quantum steerability in high-dimensional systems but also deepens the theoretical understanding of quantum steerability itself.

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• Quantum correlations, foundations & formalism
• Quantum information theory
• Machine learning