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Photoelectron spectroscopy of doubly excited helium dressed with strong near-infrared laser fields
Phys. Rev. A 114, 013105 – Published 7 July, 2026
DOI: https://doi.org/10.1103/d8qn-8y4v
Abstract
We report time-resolved photoelectron spectroscopy of the doubly excited states of helium dressed by a strong near-infrared (NIR) laser field. Using synchronized XUV free-electron-laser and 800-nm NIR laser pulses, we observe a pronounced delay-dependent shift of resonance-related spectral minima together with the emergence of additional structures around the NIR sideband energy. Ab initio theoretical calculations support these observations and identify the features as signatures of NIR-induced coupling of the bright autoionizing state to nearby dark resonances below the threshold. A multichannel Fano resonance analysis of the measured spectra yields delay-dependent line-shape parameters and resonance energies, establishing a quantitative route to characterize and control correlated two-electron resonances in strong laser fields.