- Open Access
Loss of integrability in a system with two-photon interactions
Phys. Rev. A 112, 063707 – Published 5 December, 2025
DOI: https://doi.org/10.1103/c618-hql5
Abstract
Light-matter systems that exhibit two-photon interactions have emerged as powerful platforms for exploring quantum applications. In this work, we focus on the two-photon Dicke model, a system of significant experimental relevance that displays spectral collapse and undergoes a phase transition from a normal to a superradiant phase. We analyze the normal phase, where a classical limit with two degrees of freedom can be derived using a mean-field approximation. Our study presents a detailed investigation of the loss of integrability in the two-photon Dicke model, employing both quantum and classical diagnostics. These results allow us to explore various dynamical features of the system, including the onset of chaos and the existence of mixed phase-space behavior.
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References (121)
- J. P. Dowling and G. J. Milburn, Quantum technology: The second quantum revolution, Philos. Trans. R. Soc., A 361, 1655 (2003).
- A. Zeilinger, Experiment and the foundations of quantum physics, Rev. Mod. Phys. 71, S288 (1999).
- N. Gisin and R. Thew, Quantum communication, Nat. Photonics 1, 165 (2007).
- B. Swingle, G. Bentsen, M. Schleier-Smith, and P. Hayden, Measuring the scrambling of quantum information, Phys. Rev. A 94, 040302(R) (2016).
- K. A. Landsman, C. Figgatt, T. Schuster, N. M. Linke, B. Yoshida, N. Y. Yao, and C. Monroe, Verified quantum information scrambling, Nature (London) 567, 61 (2019).
- M. A. Taylor and W. P. Bowen, Quantum metrology and its application in biology, Phys. Rep. 615, 1 (2016).
- C. L. Degen, F. Reinhard, and P. Cappellaro, Quantum sensing, Rev. Mod. Phys. 89, 035002 (2017).
- L. J. Fiderer and D. Braun, Quantum metrology with quantum-chaotic sensors, Nat. Commun. 9, 1351 (2018).
- S. E. Crawford, R. A. Shugayev, H. P. Paudel, P. Lu, M. Syamlal, P. R. Ohodnicki, B. Chorpening, R. Gentry, and Y. Duan, Quantum sensing for energy applications: Review and perspective, Adv. Quantum Technol. 4, 2100049 (2021).
- V. Montenegro, C. Mukhopadhyay, R. Yousefjani, S. Sarkar, U. Mishra, M. G.A. Paris, and A. Bayat, Review: Quantum metrology and sensing with many-body systems, Phys. Rep. 1134, 1 (2025).
- S. Lloyd, Universal quantum simulators, Science 273, 1073 (1996).
- I. M. Georgescu, S. Ashhab, and F. Nori, Quantum simulation, Rev. Mod. Phys. 86, 153 (2014).
- I. I. Rabi, On the process of space quantization, Phys. Rev. 49, 324 (1936).
- I. I. Rabi, Space quantization in a gyrating magnetic field, Phys. Rev. 51, 652 (1937).
- D. Braak, Q.-H. Chen, M. T Batchelor, and E. Solano, Semi-classical and quantum Rabi models: In celebration of 80 years, J. Phys. A: Math. Theor. 49, 300301 (2016).
- R. H. Dicke, Coherence in spontaneous radiation processes, Phys. Rev. 93, 99 (1954).
- P. Kirton, M. M. Roses, J. Keeling, and E. G. Dalla Torre, Introduction to the Dicke model: From equilibrium to nonequilibrium, and vice versa, Adv. Quantum Technol. 2, 1800043 (2019).
- M. M. Roses and E. G. Dalla Torre, Dicke model, PLoS One 15, e0235197 (2020).
- D. Villaseñor, S. Pilatowsky-Cameo, J. Chávez-Carlos, M. A. Bastarrachea-Magnani, S. Lerma-Hernández, L. F. Santos, and J. G. Hirsch, Classical and quantum properties of the spin-boson Dicke model: Chaos, localization, and scarring, arXiv:2405.20381.
- M. O. Scully and M. Suhail Zubairy, Quantum Optics (Cambridge University Press, Cambridge, 1997).
- E. T. Jaynes and F. W. Cummings, Comparison of quantum and semiclassical radiation theories with application to the beam maser, Proc. IEEE 51, 89 (1963).
- J. Larson and T. Mavrogordatos, The Jaynes–Cummings Model and its Descendants (IOP Publishing, Bristol, UK, 2021), pp. 2053–2563.
- M. Tavis and F. W. Cummings, Exact solution for an -molecule—radiation-field Hamiltonian, Phys. Rev. 170, 379 (1968).
- B. M. Garraway, The Dicke model in quantum optics: Dicke model revisited, Philos. Trans. R. Soc. A 369, 1137 (2011).
- G. S. Agarwal, Vacuum-field Rabi oscillations of atoms in a cavity, J. Opt. Soc. Am. B 2, 480 (1985).
- P. Alsing and M. S. Zubairy, Collapse and revivals in a two-photon absorption process, J. Opt. Soc. Am. B 4, 177 (1987).
- R. R. Puri and R. K. Bullough, Quantum electrodynamics of an atom making two-photon transitions in an ideal cavity, J. Opt. Soc. Am. B 5, 2021 (1988).
- A. H. Toor and M. S. Zubairy, Validity of the effective Hamiltonian in the two-photon atom-field interaction, Phys. Rev. A 45, 4951 (1992).
- R. R. Puri and G. S. Agarwal, Coherent two-photon transitions in Rydberg atoms in a cavity with finite , Phys. Rev. A 37, 3879 (1988).
- K. M. Ng, C. F. Lo, and K. L. Liu, Exact eigenstates of the two-photon Jaynes-Cummings model with the counter-rotating term, Eur. Phys. J. D 6, 119 (1999).
- C Emary and R. F. Bishop, Exact isolated solutions for the two-photon Rabi Hamiltonian, J. Phys. A: Math. Gen. 35, 8231 (2002).
- C. Emary and R. F. Bishop, Bogoliubov transformations and exact isolated solutions for simple nonadiabatic Hamiltonians, J. Math. Phys. 43, 3916 (2002).
- S. N. Dolya, Quasi-exactly solvable models based on special functions, J. Math. Phys. 49, 053524 (2008).
- S. N. Dolya, Quadratic Lie algebras and quasiexact solvability of the two-photon Rabi Hamiltonian, J. Math. Phys. 50, 033512 (2009).
- D. Braak, Integrability of the Rabi model, Phys. Rev. Lett. 107, 100401 (2011).
- Q.-H. Chen, C. Wang, S. He, T. Liu, and K.-L. Wang, Exact solvability of the quantum Rabi model using Bogoliubov operators, Phys. Rev. A 86, 023822 (2012).
- I. Travěnec, Solvability of the two-photon Rabi Hamiltonian, Phys. Rev. A 85, 043805 (2012).
- A. J. Maciejewski, M. Przybylska, and T. Stachowiak, Comment on “Solvability of the two-photon Rabi Hamiltonian,” Phys. Rev. A 91, 037801 (2015).
- I. Travěnec, Reply to “Comment on ‘Solvability of the two-photon Rabi Hamiltonian’”, Phys. Rev. A 91, 037802 (2015).
- S. Felicetti, J. S. Pedernales, I. L. Egusquiza, G. Romero, L. Lamata, D. Braak, and E. Solano, Spectral collapse via two-phonon interactions in trapped ions, Phys. Rev. A 92, 033817 (2015).
- L. Duan, Y.-F. Xie, D. Braak, and Q.-H. Chen, Two-photon Rabi model: Analytic solutions and spectral collapse, J. Phys. A: Math. Theor. 49, 464002 (2016).
- R. J. Armenta Rico, F. H. Maldonado-Villamizar, and B. M. Rodriguez-Lara, Spectral collapse in the two-photon quantum Rabi model, Phys. Rev. A 101, 063825 (2020).
- J. Peng, Z. Ren, G. Guo, and G. Ju, Integrability and solvability of the simplified two-qubit Rabi model, J. Phys. A: Math. Theor. 45, 365302 (2012).
- J. Peng, Z. Ren, G. Guo, G. Ju, and X. Guo, Exact solutions of the generalized two-photon and two-qubit Rabi models, Eur. Phys. J. D 67, 162 (2013).
- A. J. Maciejewski and T. Stachowiak, A novel approach to the spectral problem in the two photon Rabi model, J. Phys. A: Math. Theor. 50, 244003 (2017).
- S. Cui, J.-P. Cao, H. Fan, and L. Amico, Exact analysis of the spectral properties of the anisotropic two-bosons Rabi model, J. Phys. A: Math. Theor. 50, 204001 (2017).
- Z. Lü, C. Zhao, and H. Zheng, Quantum dynamics of two-photon quantum Rabi model, J. Phys. A: Math. Theor. 50, 074002 (2017).
- C. F. Lo, K. L. Liu, and K. M. Ng, The multiquantum Jaynes-Cummings model with the counter-rotating terms, Europhys. Lett. 42, 1 (1998).
- D. Braak, The -photon quantum Rabi model, in Mathematical Foundations for Post-Quantum Cryptography: Crypto-Math CREST, edited by T. Takagi, M. Wakayama, N. Kunihiro, K. Tanaka, K. Kimoto, and M. Kudo (Springer Nature, Singapore, 2026), pp. 75–87.
- Z.-J. Ying, H.-H. Han, B.-J. Li, S. Felicetti, and D. Braak, Critical quantum metrology in a stabilized two-photon Rabi model, Adv. Quantum Technol. 8, e00263 (2025).
- Z.-J. Ying, Globalized nonlinear critical quantum metrology by two-photon Rabi-Stark model, Phys. Rev. A 112, 052617 (2025).
- M. I. Mazhari and Rituraj, Efficient two photon generation from an atom in a cavity, arXiv:2504.08511.
- C. F. Lo, Spectral collapse in multiqubit two-photon Rabi model, Sci. Rep. 11, 5409 (2021).
- P. Banerjee, D. Sharma, and A. B. Bhattacherjee, Enhanced photon squeezing in two-photon Dicke model, Phys. Lett. A 446, 128287 (2022).
- C. C. Gerry and J. B. Togeas, Squeezing and photon antibunching from a two-photon Dicke model, Opt. Commun. 69, 263 (1989).
- C. Emary and T. Brandes, Chaos and the quantum phase transition in the Dicke model, Phys. Rev. E 67, 066203 (2003).
- C. Emary and T. Brandes, Quantum chaos triggered by precursors of a quantum phase transition: The Dicke model, Phys. Rev. Lett. 90, 044101 (2003).
- N. Lambert, C. Emary, and T. Brandes, Entanglement and the phase transition in single-mode superradiance, Phys. Rev. Lett. 92, 073602 (2004).
- T. Brandes, Coherent and collective quantum optical effects in mesoscopic systems, Phys. Rep. 408, 315 (2005).
- T. Brandes, Excited-state quantum phase transitions in Dicke superradiance models, Phys. Rev. E 88, 032133 (2013).
- L. Garbe, I. L. Egusquiza, E. Solano, C. Ciuti, T. Coudreau, P. Milman, and S. Felicetti, Superradiant phase transition in the ultrastrong-coupling regime of the two-photon Dicke model, Phys. Rev. A 95, 053854 (2017).
- J. Peng, C. Zheng, G. Guo, X. Guo, X. Zhang, C. Deng, G. Ju, Z. Ren, L. Lamata, and E. Solano, Dark-like states for the multi-qubit and multi-photon Rabi models, J. Phys. A: Math. Theor. 50, 174003 (2017).
- A B Klimov, J Negro, R Farias, and S. M. Chumakov, Nonlinear dynamics of the two-photon Dicke model, J. Opt. B: Quantum Semiclass. Opt. 1, 562 (1999).
- C.-L. Zhai, W. Wu, C.-W. Wu, and P.-X. Chen, Stark-induced tunable phase transition in the two-photon Dicke-Stark model, Phys. Rev. A 112, 013720 (2025).
- M. M. T. Loy, Two-photon adiabatic inversion, Phys. Rev. Lett. 41, 473 (1978).
- H. Schlemmer, D. Frölich, and H. Welling, Two-photon amplification on cascade-transitions, Opt. Commun. 32, 141 (1980).
- B. Nikolaus, D. Z. Zhang, and P. E. Toschek, Two-photon laser, Phys. Rev. Lett. 47, 171 (1981).
- D. J. Gauthier, Q. Wu, S. E. Morin, and T. W. Mossberg, Realization of a continuous-wave, two-photon optical laser, Phys. Rev. Lett. 68, 464 (1992).
- M. Brune, J. M. Raimond, and S. Haroche, Theory of the Rydberg-atom two-photon micromaser, Phys. Rev. A 35, 154 (1987).
- M. Brune, J. M. Raimond, P. Goy, L. Davidovich, and S. Haroche, Realization of a two-photon maser oscillator, Phys. Rev. Lett. 59, 1899 (1987).
- M. Brune, J. M. Raimond, P. Goy, L. Davidovich, and S. Haroche, The two-photon Rydberg atom micromaser, IEEE J. Quantum Electron. 24, 1323 (1988).
- S. Stufler, P. Machnikowski, P. Ester, M. Bichler, V. M. Axt, T. Kuhn, and A. Zrenner, Two-photon Rabi oscillations in a single quantum dot, Phys. Rev. B 73, 125304 (2006).
- E. del Valle, S. Zippilli, F. P. Laussy, A. Gonzalez-Tudela, G. Morigi, and C. Tejedor, Two-photon lasing by a single quantum dot in a high- microcavity, Phys. Rev. B 81, 035302 (2010).
- P. Bertet, S. Osnaghi, P. Milman, A. Auffeves, P. Maioli, M. Brune, J. M. Raimond, and S. Haroche, Generating and probing a two-photon Fock state with a single atom in a cavity, Phys. Rev. Lett. 88, 143601 (2002).
- X.-F. Zhang, Q. Sun, Yu-Chuan Wen, W.-M. Liu, S. Eggert, and A.-C. Ji, Rydberg polaritons in a cavity: A superradiant solid, Phys. Rev. Lett. 110, 090402 (2013).
- A. Crescente, M. Carrega, M. Sassetti, and D. Ferraro, Ultrafast charging in a two-photon Dicke quantum battery, Phys. Rev. B 102, 245407 (2020).
- L. Garbe, P. Wade, F. Minganti, N. Shammah, S. Felicetti, and F. Nori, Dissipation-induced bistability in the two-photon Dicke model, Sci. Rep. 10, 13408 (2020).
- A. J. Shah, P. Kirton, S. Felicetti, and H. Alaeian, Dissipative phase transition in the two-photon Dicke model, Phys. Rev. Lett. 135, 173602 (2025).
- J. Li, R. Fazio, and S. Chesi, Nonlinear dynamics of the dissipative anisotropic two-photon Dicke model, New J. Phys. 24, 083039 (2022).
- J. Li and S. Chesi, Routes to chaos in the balanced two-photon Dicke model with qubit dissipation, Phys. Rev. A 109, 053702 (2024).
- S. Wang, S. Chen, and J. Jing, Effect of system energy on quantum signatures of chaos in the two-photon Dicke model, Phys. Rev. E 100, 022207 (2019).
- M. A. M. de Aguiar, K. Furuya, C. H. Lewenkopf, and M. C. Nemes, Chaos in a spin-boson system: Classical analysis, Ann. Phys. (NY) 216, 291 (1992).
- L. Bakemeier, A. Alvermann, and H. Fehske, Dynamics of the Dicke model close to the classical limit, Phys. Rev. A 88, 043835 (2013).
- M. A. Bastarrachea-Magnani, S. Lerma-Hernández, and J. G. Hirsch, Comparative quantum and semiclassical analysis of atom-field systems. I. Density of states and excited-state quantum phase transitions, Phys. Rev. A 89, 032101 (2014).
- M. A. Bastarrachea-Magnani, S. Lerma-Hernández, and J. G. Hirsch, Comparative quantum and semiclassical analysis of atom-field systems. II. Chaos and regularity, Phys. Rev. A 89, 032102 (2014).
- M. A. Bastarrachea-Magnani, B. L. del Carpio, S. Lerma-Hernández, and J. G. Hirsch, Chaos in the Dicke model: Quantum and semiclassical analysis, Phys. Scr. 90, 068015 (2015).
- J. Chávez-Carlos, M. A. Bastarrachea-Magnani, S. Lerma-Hernández, and J. G. Hirsch, Classical chaos in atom-field systems, Phys. Rev. E 94, 022209 (2016).
- A. D. Ribeiro, M. A. M. de Aguiar, and A. F. R. de Toledo Piza, The semiclassical coherent state propagator for systems with spin, J. Phys. A: Math. Gen. 39, 3085 (2006).
- A. Peres, New conserved quantities and test for regular spectra, Phys. Rev. Lett. 53, 1711 (1984).
- M. Feingold, N. Moiseyev, and A. Peres, Classical limit of quantum chaos, Chem. Phys. Lett. 117, 344 (1985).
- M. Feingold and A. Peres, Distribution of matrix elements of chaotic systems, Phys. Rev. A 34, 591 (1986).
- E. Ott, Chaos in Dynamical Systems (Cambridge University Press, Cambridge, 2002).
- G. Casati, F. Valz-Gris, and I. Guarnieri, On the connection between quantization of nonintegrable systems and statistical theory of spectra, Lett. Nuovo Cimento 28, 279 (1980).
- O. Bohigas, M. J. Giannoni, and C. Schmit, Characterization of chaotic quantum spectra and universality of level fluctuation laws, Phys. Rev. Lett. 52, 1 (1984).
- F. Haake, Quantum Signatures of Chaos (Springer-Verlag, Berlin, 1991).
- H.-J. Stöckmann, Quantum Chaos: An Introduction (Cambridge University Press, Cambridge, 2006).
- S. Wimberger, Nonlinear Dynamics and Quantum Chaos (Springer International Publishing, Switzerland, 2014).
- M. C. Gutzwiller, Chaos in Classical and Quantum Mechanics (Springer-Verlag, New York, 1990).
- T. A. Brody, J. Flores, J. B. French, P. A. Mello, A. Pandey, and S. S. M. Wong, Random-matrix physics: Spectrum and strength fluctuations, Rev. Mod. Phys. 53, 385 (1981).
- T. Guhr, A. Müller-Groeling, and H. A. Weidenmüller, Random matrix theories in quantum physics: Common concepts, Phys. Rep. 299, 189 (1998).
- Y. Fyodorov, Random matrix theory, Scholarpedia 6, 9886 (2011).
- M. L. Mehta, Random Matrices (Academic Press, Boston, 1991).
- M. V. Berry, M. Tabor, and J. Michael Ziman, Level clustering in the regular spectrum, Proc. Roy. Soc. London. A. Math. Phys. Sci. 356, 375 (1977).
- V. Oganesyan and D. A. Huse, Localization of interacting fermions at high temperature, Phys. Rev. B 75, 155111 (2007).
- Y. Y. Atas, E. Bogomolny, O. Giraud, and G. Roux, Distribution of the ratio of consecutive level spacings in random matrix ensembles, Phys. Rev. Lett. 110, 084101 (2013).
- M. V. Berry and M. Robnik, Semiclassical level spacings when regular and chaotic orbits coexist, J. Phys. A: Math. Gen. 17, 2413 (1984).
- M. Robnik, Topics in quantum chaos of generic systems, Nonlinear Phenom. Complex Syst. 1, 1 (1998).
- M. Robnik, Recent developments in quantum chaos of mixed-type systems: A mini review, Nonlinear Phenom. Complex Syst. 26, 209 (2023).
- T. W. Anderson and D. A. Darling, Asymptotic theory of certain “goodness of fit” criteria based on stochastic processes, Ann. Math. Stat. 23, 193 (1952).
- B. Batistić and M. Robnik, Semiempirical theory of level spacing distribution beyond the Berry–Robnik regime: Modeling the localization and the tunneling effects, J. Phys. A: Math. Theor. 43, 215101 (2010).
- B. Batistić and M. Robnik, Dynamical localization of chaotic eigenstates in the mixed-type systems: Spectral statistics in a billiard system after separation of regular and chaotic eigenstates, J. Phys. A: Math. Theor. 46, 315102 (2013).
- B. Batistić and M. Robnik, Quantum localization of chaotic eigenstates and the level spacing distribution, Phys. Rev. E 88, 052913 (2013).
- S. Pilatowsky-Cameo, D. Villaseñor, M. A. Bastarrachea-Magnani, S. Lerma-Hernández, L. F. Santos, and J. G. Hirsch, Ubiquitous quantum scarring does not prevent ergodicity, Nat. Commun. 12, 852 (2021).
- D. Villaseñor, S. Pilatowsky-Cameo, M. A. Bastarrachea-Magnani, S. Lerma-Hernández, L. F. Santos, and J. G. Hirsch, Chaos and thermalization in the spin-boson Dicke model, Entropy 25, 8 (2023).
- M. A. Bastarrachea-Magnani, D. Villaseñor, J. Chávez-Carlos, S. Lerma-Hernández, L. F. Santos, and J. G. Hirsch, Quantum multifractality as a probe of phase space in the Dicke model, Phys. Rev. E 109, 034202 (2024).
- A. K. Das, C. Cianci, D. G. A. Cabral, D. A. Zarate-Herrada, P. Pinney, S. Pilatowsky-Cameo, A. S. Matsoukas-Roubeas, V. S. Batista, A. del Campo, E. J. Torres-Herrera, and L. F. Santos, Proposal for many-body quantum chaos detection, Phys. Rev. Res. 7, 013181 (2025).
- I. Vallejo-Fabila, A. K. Das, S. Choudhury, and L. F. Santos, Single-site measurements as probes of many-body quantum chaos, Phys. Rev. E 112, 044208 (2025).
- F. T. Arecchi, E. Courtens, R. Gilmore, and H. Thomas, Atomic coherent states in quantum optics, Phys. Rev. A 6, 2211 (1972).
- W.-M. Zhang, D. H. Feng, and R. Gilmore, Coherent states: Theory and some applications, Rev. Mod. Phys. 62, 867 (1990).
- M. A. Bastarrachea-Magnani and J. G. Hirsch, Efficient basis for the Dicke model: I. Theory and convergence in energy, Phys. Scr. 2014, 014005 (2014).
- J. G. Hirsch and M. A. Bastarrachea-Magnani, Efficient basis for the Dicke model: II. Wave function convergence and excited states, Phys. Scr. 2014, 014018 (2014).