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Magnetic Feshbach resonances in ultracold atom-molecule collisions

Masato Morita1, Maciej B. Kosicki2, Piotr S. Żuchowski3, Paul Brumer1, and Timur V. Tscherbul4

Phys. Rev. A 110, L021301 – Published 14 August, 2024

DOI: https://doi.org/10.1103/PhysRevA.110.L021301

Abstract

We report numerically exact quantum scattering calculations on magnetic Feshbach resonances in ultracold, strongly anisotropic atom-molecule [Rb(S2) + SrF(2Σ+)] collisions based on state-of-the-art ab initio potential energy surfaces. We find broad resonances mediated by the intermolecular spin-exchange interaction, as well as narrow resonances due to the intramolecular spin-rotation interaction, which are unique to atom-molecule collisions. Remarkably, the density of resonances in atom-molecule collisions is not much higher than that in atomic collisions despite the presence of a dense manifold of molecular rotational states, which can be rationalized by analyzing the adiabatic states of the collision complex.

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