- Letter
Phase dependence of resonant and antiresonant two-photon excitations
Phys. Rev. A 105, L011101 – Published 18 January, 2022
DOI: https://doi.org/10.1103/PhysRevA.105.L011101
Abstract
Measurements of the phase of two-photon matrix elements are presented for resonant and antiresonant two-color ionization of helium. A tunable, narrow-bandwidth, near-infrared (NIR) laser source is used for extreme ultraviolet (XUV) high-harmonic generation (HHG). The 15th harmonic of the laser is used within () two-photon ionization and tuned in and out of resonance with members of the () Rydberg series, covering a broad spectral range with high spectral resolution. The technique allows us to observe characteristic rapid changes in the phase of the two-photon matrix elements around the resonances and at the antiresonances between the resonances. Similar effects are observed for () three-photon ionization. The experimental results are compared to a perturbative model and to numerical solutions of the time-dependent Schrödinger equation in the single-active-electron approximation, elucidating the origin and dependences of the observed phenomena.