Export citation

Export citation

Choose format for download:

Download Citation
  • Letter

Phase dependence of resonant and antiresonant two-photon excitations

L. Drescher*, T. Witting, O. Kornilov, and M. J. J. Vrakking

  • Max-Born-Institut für nichtlineare Optik und Kurzzeitspektroskopie, Max-Born-Strasse 2A, 12489 Berlin, Germany

  • *Present address: Department of Chemistry, University of California, Berkeley, California 94720, USA; lbdrescher@berkeley.edu

Phys. Rev. A 105, L011101 – Published 18 January, 2022

DOI: https://doi.org/10.1103/PhysRevA.105.L011101

Abstract

Measurements of the phase of two-photon matrix elements are presented for resonant and antiresonant two-color ionization of helium. A tunable, narrow-bandwidth, near-infrared (NIR) laser source is used for extreme ultraviolet (XUV) high-harmonic generation (HHG). The 15th harmonic of the laser is used within (1+1′) XUV+NIR two-photon ionization and tuned in and out of resonance with members of the 1snpP11 (n=3,4,5) Rydberg series, covering a broad spectral range with high spectral resolution. The technique allows us to observe characteristic rapid changes in the phase of the two-photon matrix elements around the resonances and at the antiresonances between the resonances. Similar effects are observed for (1+2′) XUV+NIR three-photon ionization. The experimental results are compared to a perturbative model and to numerical solutions of the time-dependent Schrödinger equation in the single-active-electron approximation, elucidating the origin and dependences of the observed phenomena.

Physics Subject Headings (PhySH)

Authorization Required

We need you to provide your credentials before accessing this content.

Supplemental Material (Subscription Required)

References (Subscription Required)

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation