Parity-time ($\mathcal{PT}$)-symmetric systems, featuring real eigenvalues despite their non-Hermitian nature, undergo spontaneous $\mathcal{PT}$ symmetry breaking at the exceptional point (EP). The phase transition from $\mathcal{PT}$ symmetry to $\mathcal{PT}$ symmetry breaking has shown exotic functionalities in the classical realm, such as loss-induced transparency or lasing revival. This transition is also expected to produce a more unconventional effect in pure quantum $\mathcal{PT}$ devices. Here, we report experimental evidences of spontaneous $\mathcal{PT}$ symmetry breaking in a single cold ${}^{40}\mathrm{Ca}^{+}$ ion and, more importantly, a counterintuitive effect of perfect quantum coherence occurring at the EP. Excellent agreement between experimental results and theoretical predictions is identified. In view of the versatile role of cold ions in building a quantum memory or processor, our experiment provides an alternative platform to explore $\mathcal{PT}$-symmetric physics and utilize pure quantum EP effects.

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• PT-symmetric quantum mechanics
• Quantum information with trapped ions
• Quantum simulation
• Quantum tomography
• Resource theories