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  • Open Access

Quantum open system description of a hybrid plasmonic cavity

Marco Vallone*

  • Dipartimento di Elettronica e Telecomunicazioni, Politecnico di Torino, Corso Duca degli Abruzzi 24, 10129 Torino, Italy

  • *Contact author: marco.vallone@polito.it

Phys. Rev. A 113, 033723 – Published 16 March, 2026

DOI: https://doi.org/10.1103/2xfb-jcgy

Abstract

We present a unified quantum open system framework for lossy plasmonic cavities, treating coherent dynamics, relaxation, dephasing, and irreversible absorption on an equal footing. The Dyson equation for the cavity photon propagator in the random-phase approximation yields a complex self-energy S(ω) that accounts for both the renormalization and damping of hybrid plasmon-photon modes. It shows that increasing losses can drive a crossover from resolvable normal-mode splitting to a regime without resolved splitting, when the damping becomes comparable to or larger than the coherent hybridization scale. Tracing out the environment yields a Liouvillian for the upper polaritons (UPs) and lower polaritons (LPs) with leakage Γ=−2ImS(ω), internal UP ↔ LP scattering, and dephasing. Closed-form dynamics for populations and interbranch coherence provide analytic steady-state values, line shapes, and UP-LP quench rates, valid at low polariton density and in the ultrastrong-coupling regime. The theory is directly applicable to spectra, time-domain probes, and dissipation engineering in plasmonic and nanophotonic cavities.

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References (57)

  1. H. Raether, Surface Plasmons on Smooth and Rough Surfaces and on Gratings, Springer Tracts in Modern Physics, Vol. 111 (Springer, Berlin, 1988).
  2. E. Ozbay, Plasmonics: Merging photonics and electronics at nanoscale dimensions, Science 311, 189 (2006).
  3. S. A. Maier, Plasmonics: Fundamentals and Applications (Springer, New York, 2007).
  4. J. J. Hopfield, Theory of the contribution of excitons to the complex delectric constant of crystals, Phys. Rev. 112, 1555 (1958).
  5. H. A. Atwater and A. Polman, Plasmonics for improved photovoltaic devices, Nat. Mater. 9, 205 (2010).
  6. P. Berini, Surface plasmon–photodetectors and their applications, Laser Photonics Rev. 8, 197 (2014).
  7. J. Anker, W. P. Hall, O. O. Lyandres, N. C. Shah, J. Zhao, and R. P. V. Duyne, Biosensing with plasmonic nanosensors, Nat. Mater. 7, 442 (2008).
  8. J. Homola, S. S. Yee, and G. Gauglitz, Surface plasmon resonance sensors: Review, Sens. Actuat. B 54, 3 (1999).
  9. K. R. Catchpole and A. Polman, Plasmonic solar cells, Opt. Express 16, 21793 (2008).
  10. A. Polman and H. Atwater, Photonic design principles for ultrahigh-efficiency photovoltaics, Nat. Mater. 11, 174 (2012).
  11. S. Sarkar and T. A. F. König, Engineering plasmonic hybridization toward advanced optical sensors, Adv. Sens. Res. 3, 2300054 (2024).
  12. C. Cohen-Tannoudji, J. Dupont-Roc, and G. Grynberg, Atom-Photon Interactions: Basic Processes and Applications (Wiley, New York, 1992), p. 656.
  13. E. T. Jaynes and F. W. Cummings, Comparison of quantum and semiclassical radiation theories with application to the beam maser, Proc. IEEE 51, 89 (1963).
  14. J. Liu and Z.-Y. Li, Interaction of a two-level atom with single-mode optical field beyond the rotating wave approximation, Opt. Express 22, 28671 (2014).
  15. J. Larson and T. Mavrogordatos, The Jaynes-Cummings Model and its Descendants: Modern Research Directions, 2nd ed. (IOP, Bristol, 2024).
  16. I. I. Rabi, On the process of space quantization, Phys. Rev. 49, 324 (1936).
  17. I. I. Rabi, Space quantization in a gyrating magnetic field, Phys. Rev. 51, 652 (1937).
  18. C. Ciuti, G. Bastard, and I. Carusotto, Quantum vacuum properties of the intersubband cavity polariton field, Phys. Rev. B 72, 115303 (2005).
  19. P. Forn-Díaz, L. Lamata, E. Rico, J. Kono, and E. Solano, Ultrastrong coupling regimes of light-matter interaction, Rev. Mod. Phys. 91, 025005 (2019).
  20. A. F. Kockum, A. Miranowicz, S. D. Liberato, S. Savasta, and F. Nori, Ultrastrong coupling between light and matter, Nat. Rev. Phys. 1, 19 (2019).
  21. D. G. Baranov, B. Munkhbat, E. Zhukova, A. Bisht, A. Canales, B. Rousseaux, G. Johansson, T. J. Antosiewicz, and T. Shegai, Ultrastrong coupling between nanoparticle plasmons and cavity photons at ambient conditions, Nat. Commun. 11, 2715 (2020).
  22. M. Vallone, M. Goano, and A. Tibaldi, High operating temperature HgCdTe coupled cavity plasmonic infrared photodetectors, Opt. Express 32, 27536 (2024).
  23. M. Vallone, Renormalized photon propagator in quantum electrodynamics of plasmonic cavities, New J. Phys. 27, 064102 (2025).
  24. J.-S. Huang, V. Callegari, P. Geisler, C. Brüning, J. Kern, J. C. Prangsma, X. Wu, T. Feichtner, J. Ziegler, P. Weinmann, M. Kamp, A. Forchel, P. Biagioni, U. Sennhauser, and B. Hecht, Atomically flat single-crystalline gold nanostructures for plasmonic nanocircuitry, Nat. Commun. 1, 150 (2010).
  25. L. Liu, A. V. Krasavin, J. Zheng, Y. Tong, P. Wang, X. Wu, B. Hecht, C. Pan, J. Li, L. Li, X. Guo, A. V. Zayats, and L. Tong, Atomically smooth single-crystalline platform for low-loss plasmonic nanocavities, Nano Lett. 22, 1786 (2022).
  26. A. S. Baburin, A. I. Ivanov, E. S. Lotkov, O. S. Sorokina, I. A. Boginskaya, E. V. Sergeev, K. A. Buzaverov, T. G. Konstantinova, D. O. Moskalev, Z. Issabayeva, I. A. Ryzhikov, and I. A. Rodionov, Epitaxial silver films morphology and optical properties evolution over two years, Coatings 10, 911 (2020).
  27. T. Guo and C. Argyropoulos, Hybrid graphene-plasmon gratings, J. Appl. Phys. 134, 050901 (2023).
  28. A. Rawashdeh, A. Wildenborg, E. Liu, Z. Gao, D. A. Czaplewski, H. Qu, J. Y. Suh, and A. Yang, High-quality surface plasmon polaritons in large-area sodium nanostructures, Nano Lett. 23, 469 (2023).
  29. A. Ghorashi, N. Rivera, B. Shi, R. Sundararaman, E. Kaxiras, J. Joannopoulos, and M. Soljačić, Highly confined, low-loss plasmonics based on two-dimensional solid-state defect lattices, Phys. Rev. Mater. 8, L011001 (2024).
  30. C. Qin, B. Wang, H. Huang, H. Long, K. Wang, and P. Lu, Low-loss plasmonic supermodes in graphene multilayers, Opt. Express 22, 25324 (2014).
  31. A. Asadi, Design of multilayer graphene metamaterials plasmonic waveguides with ultra-low-loss mid-infrared, Optik 327, 172327 (2025).
  32. H.-P. Breuer and F. Petruccione, The Theory of Open Quantum Systems (Oxford University Press, Oxford, 2007).
  33. G. Lindblad, On the generators of quantum dynamical semigroups, Commun. Math. Phys. 48, 119 (1976).
  34. V. Gorini, A. Kossakowski, and E. C. G. Sudarshan, Completely positive dynamical semigroups of N‐level systems, J. Math. Phys. 17, 821 (1976).
  35. T. Hümmer, F. J. García-Vidal, L. Martín-Moreno, and D. Zueco, Weak and strong coupling regimes in plasmonic QED, Phys. Rev. B 87, 115419 (2013).
  36. B. Huttner and S. M. Barnett, Quantization of the electromagnetic field in dielectrics, Phys. Rev. A 46, 4306 (1992).
  37. S. Scheel and S. Y. Buhmann, Macroscopic quantum electrodynamics—Concepts and applications, Acta Phys. Slovaca 58, 675 (2008).
  38. F. Beaudoin, J. M. Gambetta, and A. Blais, Dissipation and ultrastrong coupling in circuit QED, Phys. Rev. A 84, 043832 (2011).
  39. S. R. K. Rodriguez, A. Abass, B. Maes, O. T. A. Janssen, G. Vecchi, and J. Gómez Rivas, Coupling bright and dark plasmonic lattice resonances, Phys. Rev. X 1, 021019 (2011).
  40. A. Canales, T. Karmstrand, D. G. Baranov, T. J. Antosiewicz, and T. O. Shegai, Polaritonic linewidth asymmetry in the strong and ultrastrong coupling regime, Nanophotonics 12, 4073 (2023).
  41. Y. Todorov and C. Sirtori, Intersubband polaritons in the electrical dipole gauge, Phys. Rev. B 85, 045304 (2012).
  42. N. S. Mueller, Y. Okamura, B. G. M. Vieira, S. Juergensen, H. Lange, E. B. Barros, F. Schulz, and S. Reich, Deep strong light-matter coupling in plasmonic nanoparticle crystals, Nature (London) 583, 780 (2020).
  43. Z. Wang, L. Li, S. Wei, X. Shi, J. Xiao, Z. Guo, W. Wang, Y. Wang, and W. Wang, Manipulating light-matter interaction into strong coupling regime for photon entanglement in plasmonic lattices, J. Appl. Phys. 133, 063101 (2023).
  44. E. A. Power and S. Zienau, On the radiative contributions to the Van der Waals force, Nuovo Cimento 6, 7 (1957).
  45. R. G. Woolley and C. A. Coulson, Molecular quantum electrodynamics, Proc. R. Soc. London A 321, 557 (1971).
  46. A. Vukics, G. Konya, and P. Domokos, The gauge-invariant Lagrangian, the Power-Zienau-Woolley picture, and the choices of field momenta in nonrelativistic quantum electrodynamics, Sci. Rep. 11, 16337 (2021).
  47. R. L. Olmon, B. Slovick, T. W. Johnson, D. Shelton, S.-H. Oh, G. D. Boreman, and M. B. Raschke, Optical dielectric function of gold, Phys. Rev. B 86, 235147 (2012).
  48. D. Yoo, F. de León-Pérez, I.-H. Lee, D. A. Mohr, M. B. Raschke, J. D. Caldwell, L. Martín-Moreno, and S. H. Oh, Ultrastrong plasmon–phonon coupling via epsilon-near-zero nanocavities, Nat. Photon. 15, 125 (2021).
  49. Z. Xi, Y. Lu, W. Yu, P. Yao, P. Wang, and H. Ming, Strong coupling between plasmonic Fabry-Pérot cavity mode and magnetic plasmon, Opt. Lett. 38, 1591 (2013).
  50. P. Törmä and W. L. Barnes, Strong coupling between surface plasmon polaritons and emitters: A review, Rep. Prog. Phys. 78, 013901 (2015).
  51. M. E. Peskin and D. V. Schroeder, Quantum Field Theory (CRC, Boca Raton, FL, 1995).
  52. Z. Rukelj and V. Despoja, Estimation of the single-particle band gap and exciton binding energy in two dimensional insulators: A modified G0W0-BSE method approach, New J. Phys. 22, 063052 (2020).
  53. S. Hughes, C. Gustin, and F. Nori, Reconciling quantum and classical spectral theories of ultrastrong coupling: role of cavity bath coupling and gauge corrections, Opt. Quantum 2, 133 (2024).
  54. N. W. Ashcroft and N. D. Mermin, Solid State Physics (Saunders, Philadelphia, 1976).
  55. A. Alexandrou, G. Bianchi, E. Péronne, B. Hallé, F. Boeuf, R. André, R. Romestain, and L. Si Dang, Stimulated scattering and its dynamics in semiconductor microcavities at 80 K under nonresonant excitation conditions, Phys. Rev. B 64, 233318 (2001).
  56. T. Virgili, D. Coles, A. M. Adawi, C. Clark, P. Michetti, S. K. Rajendran, D. Brida, D. Polli, G. Cerullo, and D. G. Lidzey, Ultrafast polariton relaxation dynamics in an organic semiconductor microcavity, Phys. Rev. B 83, 245309 (2011).
  57. D. Manzano, A short introduction to the Lindblad master equation, AIP Adv. 10, 025106 (2020).

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