Angle-resolved spectroscopy study of Ni-based superconductor
Phys. Rev. B 94, 024524 – Published 29 July, 2016
DOI: https://doi.org/10.1103/PhysRevB.94.024524
Abstract
We performed an angle-resolved photoemission spectroscopy study of the Ni-based superconductor . Electron and hole Fermi surface pockets are observed, but their different shapes and sizes lead to very poor nesting conditions. The experimental electronic band structure of is in good agreement with first-principles calculations after a slight renormalization (by a factor 1.1), confirming the picture of Hund's exchange-dominated electronic correlations decreasing with increasing filling of the shell in the Fe-, Co-, and Ni-based compounds. These findings emphasize the importance of Hund's coupling and -orbital filling as key tuning parameters of electronic correlations in transition-metal pnictides.